Quantum dot sensitized solar cells with efficiency over 12% based on tetraethyl orthosilicate additive in polysulfide electrolyte
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- Κηφεύς Ελευθερόπουλος
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1 Electronic Supplementary Material (ESI) for Journal of Materials Chemistry A. This journal is The Royal Society of Chemistry 2017 Supplementary Information (SI) Quantum dot sensitized solar cells with efficiency over 12% based on tetraethyl orthosilicate additive in polysulfide electrolyte Juan Yu, ab Wenran Wang, a Zhenxiao Pan, b Jun Du, a Zhenwei Ren, a Weinan Xue a and Xinhua Zhong* ab a Key Laboratory for Advanced Materials, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai , China b College of Materials and Energy, South China Agricultural University, 483 Wushan Road, Guangzhou , China *Corresponding author zhongxh@ecust.edu.cn
2 Fig. S1 J V curves of ZCISe based QDSCs with (6 vol%) and without Na 2 SiO 3 in the modified polysulfide electrolyte under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). Table S1 Individual photovoltaic parameters of ZCISe based QDSCs with (6 vol%) and without Na 2 SiO 3 in the modified polysulfide electrolyte under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). Na 2 SiO 3 Concentration (vol%) V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.589± ± ± ± Average 0.615± ± ± ±0.05
3 Fig. S2 J V curves of ZCISe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ).
4 Table S2 Individual photovoltaic parameters of ZCISe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). TEOS Concentration (vol%) V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.589± ± ± ± Average 0.616± ± ± ± Average 0.628± ± ± ± Average 0.615± ± ± ±0.05
5 Fig. S3 J-V curves of CdSe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ).
6 Table S3 Individual photovoltaic parameters of CdSe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). TEOS Concentration (vol%) 0 V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.648± ± ± ± Average 0.663± ± ± ± Average 0.664± ± ± ± Average 0.658± ± ± ±0.07
7 Fig. S4 J V curves of CdSeTe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ).
8 Table S4 Individual photovoltaic parameters of CdSeTe based QDSCs with different TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). TEOS Concentration (vol%) 0 V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.671± ± ± ± Average 0.695± ± ± ± Average 0.703± ± ± ± Average 0.684± ± ± ±0.05
9 Fig. S5 J V curves of ZCISe based QDSCs with 6 vol% TEOS in the modified polysulfide electrolyte at staying time of 0, 3, 12, 24 and 48 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ).
10 Table S5 Individual photovoltaic parameters of ZCISe based QDSCs with 6 vol% TEOS in the modified polysulfide electrolyte at staying time of 0, 3, 12, 24 and 48 h under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). Time (h) V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.583± ± ± ± Average 0.607± ± ± ± Average 0.625± ± ± ± Average 0.628± ± ± ± Average 0.619± ± ± ±0.07
11 Fig. S6 J-V curves of ZCISe based QDSCs with 0 and 6 vol% TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h, applying Ti mesh supported mesoporous carbon (MC/Ti) counter electrodes under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). Table S6 Impedance Individual photovoltaic parameters of ZCISe based QDSCs with 0 and 6 vol% TEOS concentrations in the modified polysulfide electrolyte at staying time of 24 h, applying Ti mesh supported mesoporous carbon (MC/Ti) counter electrodes under the illumination of 1 full sun intensity (AM 1.5G, 100 mw/cm 2 ). TEOS Concentration (v%) 0 V oc (V) J sc (ma cm -2 ) FF PCE (%) Average 0.743± ± ± ± Average 0.768± ± ± ±0.21
12 Table S7 Impedance parameters under the forward bias of 0.6 V. series resistance R s, recombination resistance R rec, chemical capacitance C μ, and electron lifetime τ n = R rec C μ. TEOS (vol%) R s W cm 2 R rec W cm 2 C μ mf cm -2 τ n ms Fig. S7 Conductivity of electrolytes containing different TEOS volumetric fractions at 25 o C.
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