Seasonal trends of atmospheric PAHs in five Asian megacities and source detection using suitable biomarkers
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- Πολωνα Μπουκουβαλαίοι
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1 1 2 3 Supporting information: Seasonal trends of atmospheric PAHs in five Asian megacities and source detection using suitable biomarkers Mahua Saha 1, Dusmant Maharana 1, Rina Kurumisawa 2, Hideshige Takada 2, Geok Bee Yeo 2, Andrea C. Rodrigues 1, BadalBhattacharya 3, Hidetoshi Kumata 4, Tomoaki Okuda 5, Kebin He 6, Yongliang Ma 6,Fumiyuki Nakajima 7, Mohamad Pauzi Zakaria 8, Duong Hoang Giang 9, Pham Hung Viet 9 1 Chemical Oceanography Division, CSIR-National Institute of Oceanography, Dona Paula, Goa , India 2 Laboratory of Organic Geochemistry, Tokyo University of Agriculture and Technology, Fuchu, Tokyo , Japan 3 Institute of Ecotoxicology and Environmental Sciences, Salt Lake, Kolkata , West Bengal, India 4 Tokyo University of Pharmacy and Life Sciences, Horinouchi, Hachioji, Tokyo , Japan 5 Department of Applied Chemistry, Faculty of Science and Technology, Keio University, Hiyoshi, Kohoku-ku, Yokohama , Japan 6 School of Environment, Tsinghua University, Beijing , China 7 The University of Tokyo, Hongo, Bunkyo-ku, Tokyo , Japan 8 Department of Environmental Sciences, Faculty of Environmental Studies, Universiti Putra Malaysia, UPM, Serdang, Selangor Darul Ehsan, Malaysia. 9 Research Center for Environmental Technology and Sustainable Development, Hanoi University of Science, Hanoi, Vietnam 1
2 Table S1 Sampling Information on Air samples on preliminary survey in Asia City (district) Sampe code Sampling date Air Temperature TSP* Location type (ºC) (µg/m 3 ) Cordinate Japan Fuchu Tokyo (summer) Jul. 31, University Campus N E Japan Fuchu Tokyo (winter) Nov. 20, University Campus N E India Kolkata Circular Road Dec.9th, Roadside N E India Kolkata Park circus Dec.11th, Roadside N E Malaysia Klang Klang Jul. 20, 2004 ~30 45 Roadside N E Malaysia Kuala Lumpur KL-center Jul. 21, 2004 ~30 80 Roadside N E Vitenam Ho Chi Minh City HCMC-1 May 17, 2004 ~ Roadside not available not available Vitenam Ho Chi Minh City HCMC-2 May 18, 2004 ~ Roadside N E Cambodia Kratie Kratie Sep. 9, 2004 ~30 64 Remote site N E Cambodia Phnom Penh Phnom Penh Sep.11, 2004 ~30 87 Roadside N E *Total suspended particles
3 Table S2. Distribution of PAHs in series of PUFs and Particles in air sample collected by High-volume air sampler* Concentration of PAH (ng/m 3 ) Series of PUF Gas** Particulates*** Total**** 1st 2nd 3rd 4th Phe Anth MP MP MP MP Fluo Pyr BaA n.d. n.d. n.d. n.d. n.d Chry 0.34 n.d. n.d. n.d BbF n.d. n.d. n.d. n.d. n.d BF n.d. n.d. n.d. n.d. n.d BeP n.d. n.d. n.d. n.d. n.d BaP n.d. n.d. n.d. n.d. n.d Pery n.d. n.d. n.d. n.d. n.d IndPy n.d. n.d. n.d. n.d. n.d BghiP n.d. n.d. n.d. n.d. n.d Cor n.d. n.d. n.d. n.d. n.d % PAH in individual PUFs 1st 2nd 3rd 4th Phe Anth MP MP MP MP Fluo Pyr BaA n.d. n.d. n.d. n.d. Chry 100 n.d. n.d. n.d. BbF n.d. n.d. n.d. n.d. BF n.d. n.d. n.d. n.d. BeP n.d. n.d. n.d. n.d. BaP n.d. n.d. n.d. n.d. Pery n.d. n.d. n.d. n.d. IndPy n.d. n.d. n.d. n.d. BghiP n.d. n.d. n.d. n.d. Cor n.d. n.d. n.d. n.d. *Air sample was collected at FS Tama of TUAT, Tokyo, Japan on Aug.4th - 5th (20 hours), 1999; AverageAir temperature : 27 o C **Sum of concentrations of PAHs in 1st to 4th PUF ***PAHs in particles collected on quartz filter (Pallflex membrane filter 2500QAT-UP) ****sum of concentrations of PAHs in gas and particulate phases
4 Table S3. PAH concentrations (ng/m 3 ) in particulate and gas phases in air samples collecte from Asian countries Japan Tokyo (summer) Tokyo (winter) Gas Particulate Total %Particulate Gas Particulate Total %Particulate Phe % % Anth % % 3-MP % % 2-MP % % 9-MP % % 1-MP % % Fluo % % Pyr % % BaA % % Chry % % BbF % % BF % % BeP % % BaP % % Pery % % IndPy % % BghiP % % Cor % % T-PAH % % 12 PAHs % % HMW-PAHs % % India Circular Road Park circus Gas Particulate Total %Particulate Gas Particulate Total %Particulate Phe % % Anth % % 3-MP % % 2-MP % % 9-MP % % 1-MP % % Fluo % % Pyr % % BaA % % Chry % % BbF % % BF % % BeP % % BaP % % Pery % % IndPy % % BghiP % % Cor % % T-PAH % % 12 PAHs % % HMW-PAHs % %
5 Table S3 (cont.) Malaysia Klang KL center Gas Particulate Total %Particulate Gas Particulate Total %Particulate Phe % % Anth % % 3-MP % % 2-MP % % 9-MP % % 1-MP % % Fluo % % Pyr % % BaA % % Chry % % BbF % % BF % % BeP % % BaP % % Pery % % IndPy % % BghiP % % Cor % % T-PAH % % 12 PAHs % % HMW-PAHs % % Vietnam HCMC center 1 HCMC center 2 Gas Particulate Total %Particulate Gas Particulate Total %Particulate Phe % % Anth % % 3-MP % % 2-MP % % 9-MP % % 1-MP % % Fluo % % Pyr % % BaA % % Chry % % BbF % % BF % % BeP % % BaP % % Pery % % IndPy % % BghiP % % Cor % % T-PAH % % 12 PAHs % % HMW-PAHs % %
6 Table S3 (cont.) Cmbodia Kratie Phnom Penh Gas Particulate Total %Particulate Gas Particulate Total %Particulate Phe % % Anth % % 3-MP % % 2-MP % % 9-MP % % 1-MP % % Fluo % % Pyr % % BaA % % Chry % % BbF % % BF % % BeP % % BaP % % Pery % % IndPy % % BghiP % % Cor % % T-PAH % % 12 PAHs % % HMW-PAHs % %
7 Figure SI 1. Seasonal variation of % particulate of several PAH species (bottom) with air temperature (top). Air samples (gas and particulate phases) were collected in Fuchu campus of Tokyo University of Agriculture and Technology (TUAT) from June to November
8 Figure SI 2. PAHs profile of the five Asian metropolitan cities: (a) Tokyo, (b) Beijing, (c) Kolkata, (d) Hanoi, (e) Kuala Lumpur
9 Figure SI 3. Seasonal changes in hopane profile of aerosols from five mega cities, a) Tokyo, b) Beijing, c) Kolkata, d) Hanoi, e) Kuala Lumpur, and comparison with that in different source materials f) wood soot, g) coal soot and h) Automobile soot 4
10 Figure SI 4. Seasonal variation of C30 17α/C30 17β ratios in (a) Tokyo, (b) Beijing, (c) Kolkata, (d) Hanoi, (e) Kuala Lumpur
Distribution Characteristics of Polycyclic Aromatic Hydrocarbons and Black Carbon in Road Dusts from Typical Cities of China and India
33 4 2012 4 ENVIRONMENTAL SCIENCE Vol 33 No 4 Apr 2012 1 2 4 2 3 1 4 1 510642 2 510640 3 510640 4 510642 PAHs BC 2007 12 ~ 2009 2 GC-MS PAHs 2 30 ~ 22 2 μg g - 1 b ghi PAHs 4 85 ~ 30 5 μg g - 1 2 PAHs
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