1 Decay Scheme. 2 Nuclear Data. 2.1 α Transitions

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1 1 Decay Scheme Pu- decays 100% by alpha transitions to U-234. Most of the alpha decay populates the U-234 ground state (71.04 %) and the U-234 first excited level with energy of (28.85 %). Branching of Pu- decay by spontaneous fission is 1.85 (5)E-7 %. Le plutonium se désintègre par émission alpha vers les niveaux fondamental (71,04 %) et excité de 43,5 (28,85 %). Le nombre de désintegrations par fission spontanée est de 1,85 (5)E-7 % 2 Nuclear Data T 1/2 ( Pu ) : 87,74 (3) a T 1/2 ( 234 U ) : 2,455 (6) 10 5 a Q α ( Pu ) : 5593,20 (19) 2.1 α Transitions Probability F 100 α 0, ,94 (20) 0, ,5 α 0, ,66 (20) 0, (7) 7,5 α 0, ,43 (20) 0, α 0, ,77 (20) 0, (16) 155 α 0, ,56 (20) 0, α 0,9 4666,48 (20) 0, (5) 53 α 0,8 4741,46 (20) 0, ,5 α 0,7 4743,93 (20) 0, (22) 3400 α 0,6 4783,29 (20) 0, α 0,5 4806,91 (20) 0, (16) 89 α 0,4 5096,16 (20) 0, (23) α 0,3 5297,13 (19) 0,00292 (4) 440 α 0,2 5449,85 (19) 0,104 (3) 102 α 0,1 5549,70 (19) 28,85 (6) 1,39 α 0,0 5593,20 (19) 71,04 (6) 1 KRI /V. Chechev 1 08/06/ /1/2010

2 2.2 Gamma Transitions and Internal Conversion Coefficients P γce Multipolarity α K α L α M α T 100 γ 8,6(U) 41,82 (11) 0, (14) [E2] 630 (13) 174 (4) 863 (18) γ 1,0(U) 43,498 (1) 28,3 (8) E2 520 (11) 143,5 (29) 713 (15) γ 11,9(U) 62,70 (1) 0, (4) E1 0,320 (7) 0,0791 (16) 0,426 (9) γ 2,1(U) 99,852 (3) 0,1060 (23) E2 9,77 (20) 2,71 (6) 13,42 (27) γ 11,7(U) 140,15 (2) 0, (7) M1 63% E2 2,6 (8) 1,79 (5) 0,48 (14) 5,1 (15) γ 3,2(U) 152,719 (2) 0,00292 (4) E2 0,217 (4) 1,404 (28) 0,388 (8) 2,14 (4) γ 13,8(U) 192,91 (7) 0, (4) [E2] 0,1635 (33) 0,505 (10) 0,1391 (28) 0,856 (17) γ 4,3(U) 200,97 (3) 0, (23) E2 0,1534 (31) 0,424 (9) 0,1166 (23) 0,734 (15) γ 11,5(U) 203,12 (3) 0, (5) M1 66% E2 0,90 (17) 0,423 (9) 0,1113 (23) 1,5 (3) γ 14,8(U) 233,6 (2) 0, (E0 E2) γ 13,6(U) 234,6 (2) 0, E0 γ 14,7(U) 235,9 (3) 0, (5) [E1] 0,0532 (11) 0,01067 (21) 0,00258 (5) 0,0673 (14) γ 13,5(U) 258,227 (3) 0, (12) (E1) 0,0434 (9) 0,00859 (17) 0,00207 (4) 0,0548 (11) γ 14,5(U) 299,1 (2) 0, (3) [E1] 0,0314 (6) 0,00608 (12) 0, (29) 0,0395 (8) γ 7,2(U) 705,9 (1) 0, (13) [E1] 0,00568 (12) 0, (20) 0, (5) 0,00698 (14) γ 8,2(U) 708,3 (2) 0, (3) [E2] 0,01537 (31) 0,00489 (10) 0, (25) 0,0219 (5) γ 12,3(U) 727,8 (2) 0, (3) (E2) 0,01464 (29) 0,00454 (9) 0, (23) 0,0207 (4) γ 5,1(U) 742,813 (5) 0, (13) E1 0,00518 (10) 0, (18) 0, (4) 0,00636 (13) γ 6,1(U) 766,38 (2) 0, (5) E2 0,01336 (27) 0,00396 (8) 0, (20) 0,0187 (4) γ 9,2(U) 783,4 (1) 0, (3) [E2] 0,01285 (26) 0,00374 (8) 0, (19) 0,0179 (4) γ 5,0(U) 786,27 (3) 0, (9) E1 0,00467 (9) 0, (16) 0, (4) 0,00573 (12) γ 10,2(U) 804,4 (3) 0, E0 E2 0,57 γ 7,1(U) 805,80 (5) 0, (15) [E1] 0,00447 (9) 0, (16) 0, (4) 0,00549 (11) γ 8,1(U) 808,2 (1) 0, E0 17% E2 3,31 0,94 4,3 γ 6,0(U) 810,0 (5) 0, E0 60 γ 8,0(U) 851,7 (1) 0, (4) [E2] 0,01109 (22) 0,00302 (6) 0, (16) 0,01513 (30) γ 12,2(U) 880,5 (1) 0, (E0 E2) γ 9,1(U) 883,24 (4) 0, (4) E2 0,01040 (21) 0,00276 (6) 0, (14) 0,01409 (28) γ 10,1(U) 904,37 (15) 0, (11) [E2] 0,00998 (20) 0,00260 (5) 0, (13) 0,01346 (27) γ 9,0(U) 926,72 (1) 0, (25) (E2) 0,00956 (20) 0,00245 (5) 0, (12) 0,01284 (26) γ 14,2(U) 941,94 (10) 0, (23) [E2] 0,00929 (20) 0,00236 (5) 0, (12) 0,01244 (25) γ 11,1(U) 946,00 (3) 0, (13) (E1) 0,00337 (7) 0, (12) 0, (27) 0,00412 (8) γ 12,1(U) 980,3 (1) 0, (E2) 0,00866 (18) 0,00214 (4) 0, (11) 0,01152 (23) γ 13,1(U) 1001,03 (3) 0, (4) E2 0,00835 (17) 0,00204 (4) 0, (11) 0,01107 (22) γ 14,1(U) 1041,7 (2) 0, (E0 E2) γ 14,0(U) 1085,4 (2) 0, (9) (E2) 0,00725 (15) 0,00169 (3) 0, (8) 0,00950 (19) 3 Atomic Data 3.1 ω K : 0,970 (4) ω L : 0,500 (19) n KL : 0,794 (5) KRI /V. Chechev 2 08/06/ /1/2010

3 3.1.1 X Radiations Relative probability K Kα 2 94,666 62,47 Kα 1 98, Kβ 3 110,421 } Kβ 1 111,298 } Kβ 5 111,964 } 36,08 Kβ 2 114,407 } Kβ 4 115,012 } 12,34 KO 2,3 115,377 } L Ll 11,619 Lα 13,438 13,615 Lη 15,399 Lβ 15,727 18,206 Lγ 19,507 20, Auger Electrons Relative probability Auger K KLL 71,78 80, KLX 88,15 98,43 59,6 KXY 104,51 115,59 8,88 Auger L 5,9 21,6 4 α Emissions Probability 100 α 0, ,1 (2) 0, α 0, ,1 (2) 0, (7) α 0, ,5 (2) 0, KRI /V. Chechev 3 08/06/ /1/2010

4 Probability 100 α 0, ,3 (2) 0, (16) α 0, ,4 (2) 0, α 0,9 4587,9 (2) 0, (5) α 0,8 4661,7 (2) 0, α 0,7 4664,1 (2) 0, (22) α 0,6 4702,8 (2) 0,0001 α 0,5 4726,0 (2) 0, (16) α 0,4 5010,4 (2) 0, (23) α 0,3 5208,0 (2) 0,00292 (4) α 0,2 5358,1 (2) 0,104 (3) α 0,1 5456,3 (2) 28,85 (6) α 0,0 5499,03 (20) 71,04 (6) 5 Electron Emissions Electrons per 100 disint. e AL (U) 5,9-21,6 10,6 (4) e AK (U) 0, (15) KLL 71,78-80,95 } KLX 88,15-98,43 } KXY 104,51-115,59 } ec 1,0 L (U) 21,74-26,33 20,6 (6) ec 1,0 M (U) 37,95-39,95 5,7 (12) ec 1,0 N (U) 42,057-43,119 1,544 (39) ec 2,1 L (U) 78,095-82,685 0,0718 (17) 6 Photon Emissions 6.1 X-Ray Emissions Photons per 100 disint. XL (U) 11,619 20,714 10,63 (8) KRI /V. Chechev 4 08/06/ /1/2010

5 Photons per 100 disint. XKα 2 (U) 94,666 0, (3) } Kα XKα 1 (U) 98,440 0, (5) } XKβ 3 (U) 110,421 } XKβ 1 (U) 111,298 } 0, (22) K β 1 XKβ 5 (U) 111,964 } XKβ 2 (U) 114,407 } XKβ 4 (U) 115,012 } 0, (6) K β 2 XKO 2,3 (U) 115,377 } 6.2 Gamma Emissions Photons per 100 disint. γ 8,6 (U) 41,82 (11) 0, (16) γ 1,0 (U) 43,498 (1) 0,0397 (8) γ 11,9 (U) 62,70 (1) 0, (3) γ 2,1 (U) 99,852 (3) 0,00735 (8) γ 11,7 (U) 140,15 (2) 0, (7) γ 3,2 (U) 152,719 (2) 0, (7) γ 13,8 (U) 192,91 (7) 0, (20) γ 4,3 (U) 200,97 (3) 0, (13) γ 11,5 (U) 203,12 (3) 0, (15) γ 14,7 (U) 235,9 (3) 0, (5) γ 13,5 (U) 258,227 (3) 0, (11) γ 14,5 (U) 299,1 (2) 0, (3) γ 7,2 (U) 705,9 (1) 0, (13) γ 8,2 (U) 708,3 (2) 0, (3) γ 12,3 (U) 727,8 (2) 0, (3) γ 5,1 (U) 742,813 (5) 0, (13) γ 6,1 (U) 766,38 (2) 0, (5) γ 9,2 (U) 783,4 (1) 0, (3) γ 5,0 (U) 786,27 (3) 0, (9) γ 10,2 (U) 804,4 (3) 0, (5) γ 7,1 (U) 805,80 (5) 0, (15) γ 8,1 (U) 808,2 (1) 0, (25) γ 8,0 (U) 851,7 (1) 0, (4) γ 12,2 (U) 880,5 (1) 0, (4) γ 9,1 (U) 883,24 (4) 0, (4) γ 10,1 (U) 904,37 (15) 0, (11) γ 9,0 (U) 926,72 (1) 0, (25) γ 14,2 (U) 941,94 (10) 0, (23) γ 11,1 (U) 946,00 (3) 0, (13) KRI /V. Chechev 5 08/06/ /1/2010

6 Photons per 100 disint. γ 12,1 (U) 980,3 (1) 0, γ 13,1 (U) 1001,03 (3) 0, (4) γ 14,1 (U) 1041,7 (2) 0, (16) γ 14,0 (U) 1085,4 (2) 0, (9) 7 Main Production Modes Np 237(n,γ)Np Np (β )Pu Cm 242(α)Pu 8 References - A. H. Jaffey, A. Hirsch. Report ANL-4286 (1949) - A. H. Jaffey, J. Lerner. Report ANL-4411 (1950) - A. H. Jaffey, L. B. Magnusson. Paper No National Nuclear Plutonium Project Record Div. IV. 14B (1951) - A. H. Jaffey. Ibid. Paper No (1951) - G. T. Seaborg, R. A. James and A. Giorso. The Transuranium Elements Paper No National Nuclear Series, Plutonium Project Record, Div. IV. 14B.Part II (1951) p E. Segre. Phys. Rev. 86 (1952) 21 - K. W. Jones, R.A. Douglas, M.T. McEllistrem and H.T. Richards. Phys. Rev. 94 (1954) F. Asaro, I. Perlman. Phys. Rev. 94 (1954) E. L. Church, A. W. Sunyar. Phys. Rev. 98 (1955) 1186A (Gamma-ray energies) - J. O. Newton, B. Rose and J. Milsted. Phil. Mag. 1 (1956) 981 (Gamma-ray energies) - D. C. Hoffman, G. P. Ford and F. O. Lawrence. J. Inorg. Nucl. Chem. 5 (1957) 6 - L. N. Kondratev, G. I. Novikova, V. B. Dedov and L. L. Goldin. Izv. Akad. Nauk SSSR, Ser Fiz 21 (1957) V. A. Druin, V. P. Perelygin and G. I. Khlebnikov. Soviet Phys. JETP 13 (1961) C. F. Leang. Compt. Rend. 255 (1962) 3155 KRI /V. Chechev 6 08/06/ /1/2010

7 - S. Bjornholm, C. M. Lederer, F. Asaro and I. Perlman. Phys. Rev. 130 (1963) 2000 (Alpha transition probabilities) - C. M. Lederer. Priv Comm, quoted by 1967Le24 (1964) (E0E2 transition probabilities) - J. W. Halley, D. Engelkemeir. Phys. Rev. 134 (1964) A24 - F. Les. Acta. Phys. Polon. 26 (1964) 951 (E0E2 transition probabilities) - J. F. Eichelberger, G. R. Grove and L. V. Jones. MLM-1 (1965) (1965) - K. C. Jordan. Report No. MLM-1443, July - September 1967 (1967) - J. Byrne, W. Gelletly, M. A. S. Ross and F. Shaikh. Phys. Rev. 170 (1968) 80 - L. Salgueiro et al.,. C.R. Acad. Sci. 267B (1968) K. L. Swinth. Nucleonics in Aerospace,Ed. P. Polishuk, N.Y. Plenum PressEd. P. Polishuk, N.Y. Plenum PressEd. P. Polishuk, N.Y. Plenum Press (1968) p S. A. Baranov, V. M. Kulakov and V. M. Shatinskii. Nucl. Phys. 7 (1968) S. R. Amtey, J. H. Hamilton, A. V. Ramayya. Nucl. Phys. A126 (1969) 201 (Conversion electron relative intensities) - D. Benson. Priv. Comm. (1969). (1969) - C. M. Lederer, F. Asaro and I. Perlman. UCRL p.3 (1969) - S. A. Baranov, V. M. Kulakov, V. M. Shatinskii and Z. S. Gladkikh. Yad. Fiz. 12 (1970) J. E. Cline. IN-1448 Rev. (1971) - K. L. Swinth. IEEE Transactions Nuclear Science, part 1 18 (1971) J. C. Soares, J. P. Ribeiro, A. Goncalves, F. B. Gil and J. C. Ferreira. Compt. Rend. 273B (1971) A. I. Makarenko, L. A. Ostretsov and N. V. Forafontov. Izv.Akad.Nauk SSSR, Ser.Fiz. 35 (1971) B. Grennberg, A. Rytz. Metrologia. 7 (1971) 65 (Alpha-particle energies) - R. Gunnink, R. J. Morrow. UCRL (1971) - J. D. Hastings, W. W. Strohm. J. Inorg. Nucl. Chem. 34 (1972) 25 - M. Schmorak, C. E. Bemis Jr., M J. Zender, N. B. Gove and P. F. Dittner. Nucl. Phys. A178 (1972) 410 (Gamma-ray energies) - W. W. Strohm, K. C. Jordan. Nucl. Soc. 18 (1974) R. R. Gay, R. Sher. Bull. Am. Phys. Soc. 20(2) (1975) 160, GB13 - H. Umezawa, T. Suzuki and S. Ichikawa. J. Nucl. Sci. Technol. 13 (1976) 327 (Gamma-ray and emission probabilities) - R. Gunnink, J. E. Evans and A. L. Prindle. UCRL (1976) - D. G. Vasilik, R. W. Martin. Nucl. Instrum. Methods 135 (1976) V. G. Polyukhov, G. A. Timofeev, P. A. Privalova, V. Y. Gabeskiriya and A. P. Chetverikov. At. Energ. 40 (1976) 61 - C. E. Bemis Jr., L. Tubbs. Report ORNL-5297 (1977) (1977) 93 KRI /V. Chechev 7 08/06/ /1/2010

8 - H. Diamond, W. C. Bentley, A. H. Jaffey and K. F. Flynn. Phys. Rev. C15 (1977) F. P. Larkins. Atomic Data and Nuclear Data Tables. 20 (1977) 313 (Auger electron energies) - F. Rosel, H. M. Friess, K. Alder and H. C. Pauli. At. Data Nucl. Data Tables. 21 (1978) 92 (Theoretical ICC) - R. Vaninbroukx, G Grosse and W. Zehner. Report CBNM/RN/45/79 (1979). (1979) (Gamma-ray emission probabilities) - A. Cesana, G. Sandrelli, V. Sangiust and M. Terrani. Energia Nucl. (Milan) 26 (1979) V. D. Sevastyanov, V. P. Jarina. Voprosi Atomnoi Nauki i Tekhniki, seriya Jadernie Konstanti. 5(44) (1981) 21 - S. K. Aggarwal, A. V. Jadhav, S. A. Chitambar, K. Raghuraman, S. N. Acharya, A. R. Parab, C. K. Sivaramakrishnan and H. C. Jain. Radiochem. Radioanal. Lett. Radiochem. Radioanal. Lett. Radiochem. Radioanal. Lett. 46 (1981) 69 - G. Barreau, H. G. Borner, T. von Egidy, R. W. Hoff. Z. Phys. A308 (1982) 209 (KX-ray energies) - I. Ahmad, J. Hines, J. E. Gindler. Phys. Rev. C27 (1983) 2239 (KX-ray energies) - P. Dryak, Yu. S. Egorov, V. G. Nedovesov, I. Plkh, G. E. Shukin. Program and Theses, Proc. 34th Ann. Conf. Nucl. Spectrosc. At. Nuclei, Alma-Ata, (1984) (1984) p V. V. Ovechkin, V. M. Chesalin and I. A. Shkabura. Izv. Akad. Nauk SSSR, Ser. Fiz. 48 (1984) R. G. Helmer, C. W. Reich. Int. J. Appl. Radiat. Isotop. 35 (1984) G. Bortels, B. Denecke, R. Valninbroukx. Nucl. Instrum. Meth. 223 (1984) 329 (Alpha-particle, gamma-ray and LX-ray energies and emission probabilities) - L. M. Bak, P. Dryak, V. G. Nedovesov, S. A. Sidorenko, G. E. Shukin, K. P. Yakovlev. Program and Theses, Proc. 34th Ann. Conf. Nucl. Spectrosc. At. Nuclei, Alma-Ata (1984) p541 - I. Ahmad. Nucl. Instrum. Meth. 223 (1984) P. A. Burns, P. N. Johnston and J.R. Moroney. Priv. Comm. (1984). (1984) - G. Bortels, P. Collaers. Appl. Radiat. Isot. 38 (1987) Yu. A. Selitsky, V. B. Funshtein, V. A. Yakovlev. Program and Theses, Proc.38th Ann. Conf. Nucl. Spectrosc. Struct. At. Nuclei, Baku (1988) p Yu. S. Popov, I. B. Makarov, D. Kh. Srurov, E. A. Erin. Sov. Radiochem. 32 (1990) 425 (MX-ray emission probability) - P. N. Johnston, J. R. Moroney and P. A. Burns. Appl. Radiat. Isot. 42 (1991) 245 (Alpha-particle energies) - A. Rytz. At. Data Nucl. Data Tables. 47 (1991) 205 (Alpha-particle energies) - M. C. Lepy, B. Duchemin, J. Morel. Nucl.Instrum.Methods Phys.Res. A353 (1994) 10 (LX ray energies and emission probabilities) - D. T. Baran. Appl. Radiat. Isot. 45 (1994) 1177 (Gamma-ray emission probabilities) - P. N. Johnston, P. A. Burns. Nucl. Instrum. Meth. Phys. Res. A361 (1995) 229 (LX-ray energies and emission probabilities) - E. Schönfeld, H. Janssen. Nucl. Instrum. Meth. Phys. Res. A369 (1996) 527 (Atomic data) - J. Yang, J. Ni. Nucl. Instrum. Meth. Phys. Res. A413 (1998) E. Schönfeld, G. Rodloff. PTB (1999) (KX-ray energies and relative emission probabilities) KRI /V. Chechev 8 08/06/ /1/2010

9 - R. G. Helmer, C. van der Leun. Nucl. Instrum. Meth. Phys. Res. A450 (2000) 35 (Gamma-ray energies) - N. E. Holden, D. C. Hoffman. Pure Appl. Chem. 72 (2000) Y. Nir-El. Radiochim. Acta 88 (2000) 83 (Gamma-ray energies) - E. Schönfeld, H. Janssen. Appl. Rad. Isot. 52 (2000) 595 (LX-ray and Auger electron emission probabilities) - G. Audi, A. H. Wapstra, C. Thibault. Nucl.Phys. A729 (2003) 337 (Q value) - E. Browne, J. K. Tuli. Nuclear Data Sheets 108 (2007) 681 (Level energies and data from 234Pa and 234Np decays) - T. Kibédi, T. W. Burrows, M. B. Trzhaskovskaya, P. M. Davidson, C. W. Nestor Jr.. Nucl.Instrum.Methods Phys.Res. A589 (2008) 202 (Theoretical ICC) KRI /V. Chechev 9 08/06/ /1/2010

10 LNE-LNHB/CEA - Table de Radionucléides 0,76 ns 1,38 ps γ Emission intensities per 100 disintegrations ,000 0,000 0,000 0,000 0, ,000 0,000 0, ,00 0,00 0, ,00 0,00 0,00 0, ,00 0, ,00 0,00 0, ; 1085,26 0 ; 1044,536 4 ; 1023,77-2 ; 989,43 4 ; 947,64 2 ; 926,72 0 α 0, , , , , , Pu ; 0 Pu ,74 (3) a 1,74 ps ; 851, ; 849,266 0 ; 809,907-1 ; 786,288 0, , ,0001 0, , ; 296,072 0, ; 143,352 0,252 ns 2,455 (6) x10^5 a U α Q = 5593,2 % α = ; 43,4981 KRI / V.P. Chechev Scheme page : 1/2 08/06/ /06/ ; 0 28,85 71,04

11 LNE-LNHB/CEA - Table de Radionucléides Pu γ Emission intensities per 100 disintegrations 0 α Pu ; 0 87,74 (3) a 1,74 ps ,00 0,00 0,00 0,00 0,00 0, , ,00 0,00 2 ; 851, ; 849,266 0 ; 809,907-1 ; 786,288 0, , ,0001 0, , ; 497,04 0, , ; 296,072 0, , ; 143,352 0,104 0,252 ns 1 2,455 (6) x10^5 a 0 0, U α Q = 5593,2 % α = ; 43, ; 0 28,85 71,04 KRI / V.P. Chechev Scheme page : 2/2 08/06/ /06/2009

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