1 Decay Scheme. 2 Nuclear Data. 2.1 Electron Capture Transitions. 2.2 Gamma Transitions and Internal Conversion Coefficients

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1 1 Decay Scheme Pb- disintegrates by electron capture to Tl- via excited levels. Le plomb se désintègre par capture électronique vers des niveaux excités du thallium. 2 Nuclear Data T 1/2 ( Pb ) : 51,929 (10) h Q ( Pb ) : 975 (6) 2.1 Electron Capture Transitions Probability Nature lg ft P K P L P M 100 ɛ 0,2 294 (6) 4,80 (8) Unique 1st Forbidden 6,812 0,7076 (32) 0,2168 (22) 0,0756 (9) ɛ 0,1 696 (6) 95,20 (12) 1st Forbidden 6,404 0,7786 (4) 0,1661 (3) 0,0552 (1) 2.2 Gamma Transitions and Internal Conversion Coefficients P γce Multipolarity α K α L α M α T 100 γ 1,0(Tl) 279,1952 (10) 99,24 (9) M1 E2 0,164 (1) 0,04837 (48) 0,2261 (8) γ 2,1(Tl) 401,320 (3) 4,04 (8) M1 0,09 % E2 0,1464 (21) 0,0245 (4) 0,00572 (8) 0,1784 (25) γ 2,0(Tl) 680,515 (3) 0,765 (18) E2 0,01065 (15) 0,00250 (4) 0, (9) 0,01393 (20) LNE - LNHB /V. Chisté, M.M. Bé 1 02/05/ /9/2006

2 3 Atomic Data 3.1 Tl ω K : 0,963 (4) ω L : 0,367 (15) n KL : 0,812 (5) X Radiations Relative probability K Kα 2 70, ,24 Kα 1 72, Kβ 3 82,116 } Kβ 1 82,5756 } Kβ 5 83,0456 } 34,01 Kβ 5 83,1417 } Kβ 2 84,867 } Kβ 4 85,1357 } 10,1 KO 2,3 85,444 } L Ll 8,9531 Lα 10, ,2679 Lη 10,9942 Lβ 11, ,9566 Lγ 13, , Auger Electrons Relative probability Auger K KLL 54,587 59, KLX 66,37 72,86 55,4 KXY 78,12 85,50 7,67 Auger L 5,43 10,93 LNE - LNHB /V. Chisté, M.M. Bé 2 02/05/ /9/2006

3 4 Electron Emissions Electrons per 100 disint. e AL (Tl) 5,43-10,93 57,9 (6) e AK (Tl) 3,4 (4) KLL 54,587-59,954 } KLX 66,37-72,86 } KXY 78,12-85,50 } ec 1,0 K (Tl) 193,665 (1) 13,27 (12) ec 1,0 L (Tl) 263, ,5377 3,912 (46) ec 1,0 M (Tl) 275, ,8059 1,254 (18) ec 2,1 K (Tl) 315,790 (3) 0,502 (13) 5 Photon Emissions 5.1 X-Ray Emissions Photons per 100 disint. XL (Tl) 8, , ,2 (6) XKα 2 (Tl) 70, ,61 (19) } Kα XKα 1 (Tl) 72, ,24 (25) } XKβ 3 (Tl) 82,116 } XKβ 1 (Tl) 82,5756 } 14,70 (24) K β 1 XKβ 5 (Tl) 83,0456 } XKβ 5 (Tl) 83,1417 } XKβ 2 (Tl) 84,867 } XKβ 4 (Tl) 85,1357 } 4,37 (11) K β 2 XKO 2,3 (Tl) 85,444 } 5.2 Gamma Emissions Photons per 100 disint. γ 1,0 (Tl) 279,1952 (10) 80,94 (5) γ 2,1 (Tl) 401,320 (3) 3,43 (6) γ 2,0 (Tl) 680,515 (3) 0,754 (18) LNE - LNHB /V. Chisté, M.M. Bé 3 02/05/ /9/2006

4 6 Main Production Modes Tl (d,2n)pb Tl (p,n)pb Tl (He 3,3n)Bi Bi (E.C.)Pb Hg 202(α,3nγ)Pb Pb 205(p,t)Pb Hg 204(α,5n)Pb Hg 202(α,3n)Pb Pb 204(γ,n)Pb Pt 198(Be 9,4n)Pb 7 References - K. Fajans, A. F. Voigt. Phys. Rev. 60 (1941) 619 (Half-life (Pb-)) - R. L. Heath, P. R. Bell. Phys. Rev. 87 (1952) 176A - J. R. Prescott. Proc. Phys. Soc. (London) A67 (1954) 254 (Half-life (Pb-), gamma energy and intensities.) - S. Thulin, K. Nybö. Ark. Fysik 7 (1954) A. H. Wapstra, D. Maeder, G. J. Nijgh, L. Th. M. Ornstein. Physica 20 (1954) 169 (Conversion coefficient, E.C. branching, gamma energy and intensities.) - R. E. Azuma, G. M. Lewis. Phil. Mag. 46 (1955) R. K. Doerner, A. H. Weber. Phys. Rev. 99 (1955) 672A - N. Marty. Comp. Rend. Acad. Sci. (Paris) 240 (1955) C. Nordling, K. Siegbahn, E. Sokolowski. Nucl. Phys. 1 (1956) 326 (Conversion coefficients.) - Z. O Friel, A. H. Weber. Phys. Rev. 101 (1956) A. H. Wapstra, G. J. Nijgh. Nucl. Phys. 1 (1956) 245 (Conversion coefficients.) - J. L. Wolfson. Can. J. Phys. 34 (1956) E. E. Berlovich, G. V. Dubinkin. Soviet Phys. JETP 5 (1957) A. A. Bartlett, G. Rebka. Bull. Am.Phys. Soc. 3,2 (1958) 64 (Half-life (Pb-)) - G. J. Nijgh, A. H. Wapstra, L. Th. M. Ornstein, N. Salomons-Grobben, J. R. Huizenga. Nucl. Phys. 9 (1958) 528 (Conversion coefficients, gamma energy.) - B. I. Deutch, N. Goldberg. Phys. Rev. 117 (1960) 818 (401- mixing ratio.) - S. Gorodetzky, R. Manquenouille, R. Richert, A. Knipper. Comp. Rend. Acad. Sci. (Paris) 251 (1960) 65 - B. Johansson, T. Alväger. Ark. Fysik 17 (1960) E. C. B. Pederson, R. E. Bell. Nucl. Phys. 21 (1960) R. W. Peelle. ORNL 3016 (1960) 116 LNE - LNHB /V. Chisté, M.M. Bé 4 02/05/ /9/2006

5 - M. K. Ramaswamy, P. S. Jastram. Nucl. Phys. 15 (1960) R. Stockendal. Ark. Fysik 17 (1960) E. Bashandy, T. R. Gerholm, J. Lindskog. Ark. Fysik 17 (1960) A. Schwarzschild, J. V. Kane. Phys. Rev. 122 (1961) T. R. Gerholm, B. G. Pettersson, B. van Nooijen, Z. Grabowski. Nucl. Phys. 24 (1961) 177 (401- mixing ratio) - J. P. Hurley, J. M. Ferguson. Nucl. Phys. 27 (1961) 75 - L. Persson, Z. Sujkowski. Ark. Fysik 19 (1961) 309 (Half-life (Pb-)) - Z. Sujkowski. Ark. Fysik 20 (1961) Th. J. de Boer, H. Voorthuis, J. Blok. Physica 28 (1962) J. P. Hurley, J. M. Ferguson. Addendun: Nucl. Phys. 31 (1962) J. G. V. Taylor. Can. J. Phys. 40 (1962) R. Burmeister, H. Graber, J. Schintlmeister, R. Weibrecht. Nucl. Phys. 42 (1963) 56 - W. L. Croft, B.-G. Pettersson, J. H. Hamilton. Nucl. Phys. 48 (1963) C. J. Herrlander, R. L. Graham. Nucl. Phys. 58 (1964) 544 (401- mixing ratio, conversion coefficients, gamma energies) - R. Rougny, J. J. Samueli, A. Sarazin. J. de Physique 25 (1964) E. C. B. Pederson, R. E. Bell. Corrigendum: Nucl. Phys. 29 (1964) E. Karlsson, E. Matthias, S. Gustafsson, K. Johansson, Å. G. Svensson, S. Ogaza, P. da Rocha Andrade. Nucl. Phys. 61 (1965) 582 (401- mixing ratio.) - M. Raja Rao, S. Jnanananda. Nucl. Instrum. Meth. 35 (1965) 261 (Conversion coefficients.) - A. Walthert, E. Baumgartner, P. Huber. Helv. Phys. Acta 38 (1965) H. E. Bosch, E. Szichman, A. Baseggio, R. Dolinkue. Nucl. Instrum. Meth. 52 (1967) J. C. Palathingal, M. L. Wiedenbeck. Nucl. Phys. A101 (1967) M. S. Rajput. Current Sci. (India) 37 (1968) 639 (Conversion coefficient) - H. S. Sahota, B. S. Ghumman, B. S. Sood. Current Sci. (India) 37 (1968) 42 - J. E. Cline. IN 1130 (1969) 39 (Gamma energies) - K.F. Walz, H. M. Weiss, E. Funck. PTB Jahresbericht (1971) G. A. Chackett, K. F. Chackett, J. B. Welborn. Int. J. Appl. Radiat. Isotop. 22 (1971) 715 (Half-life (Pb-)) - H. H. Hansen, D. Mouchel. Z. Physik 267 (1974) R. G. Helmer, R. C. Greenwood, R. J. Gehrke. Nucl. Instrum. Meth. 155 (1978) 189 (Gamma energies) - H. Houtermans, O. Milosevic, F. Reichel. Int. J. Appl. Radiat. Isotop. 31 (1980) 153 (Half-life (Pb-)) LNE - LNHB /V. Chisté, M.M. Bé 5 02/05/ /9/2006

6 - D. D. Hoppes. NBS - SP 626 (1982) 85 (Half-life (Pb-)) - H. H. Hansen. European Appl. Res. Rept. Nucl. Sci. Technol. 6 (1985) Zs. Németh, T. Sekine, Y. Yoshihara. Appl. Rad. Isotopes 40 (1989) 519 (E. C. branching, gamma intensities) - E. Schönfeld, H. Janssen. Nucl. Instrum. Meth. Phys. Res. A369 (1996) 527 (Atomic data) - E. Schönfeld, H. Janssen. Appl. Rad. Isotopes 52 (2000) 955 (Conversion coefficient) - R. G. Helmer, C. van der Leun. Nucl. Instrum. Meth. Phys. Res. A450 (2000) 35 (Gamma energies) - K. Lindenberg, F. Neumann, D. Galaviz, T. Hartmann, P. Mohr, K. Vogt, S. Volz, A. Zilges. Phys. Rev. C63 (2001) (Half-life (Pb-)) - M. P. Unterweger. Appl. Rad. Isotopes 56 (2002) 125 (Half-life (Pb-)) - G. Audi, A. H. Wapstra, C. Thibault. Nucl. Phys. A729 (2003) 129 (Q) - F. G. Kondev. Nucl. Data Sheets 105 (2005) 1 (Spin, parity, multipolarity, level energy) - S. Raman, M. Ertugrul, C. W. Nestor, Jr., M. B.Trzhaskovskaya. At. Data. Nucl. Data Tables 92 (2006) 207 (Theoretical ICC) LNE - LNHB /V. Chisté, M.M. Bé 6 02/05/ /9/2006

7 LNE-LNHB/CEA - Table de Radionucléides Pb γ Emission intensities per 100 disintegrations 0 ε Pb /2 ; 0 51,929 (10) h 0,88 ps 2 4 3,43 0,75 5/2 ; 680,5164 4,8 282,3 ps 1 8 0,94 3/2 ; 279, ,2 Stable 0 Tl Q = 975 % ε = 100 1/2 ; 0 LNE - LNHB / V. Chisté, M.M. Bé Scheme page : 1/1 02/05/ /05/2006

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