1 Decay Scheme. 2 Nuclear Data. 2.1 Electron Capture Transitions. 2.2 β + Transitions
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1 1 Decay Scheme Zr- (half-life of h) undergoes 100% EC/positron decay (Q EC of (28) kev) to various nuclear levels, including the metastable and ground states of Y-. Le zirconium se désintègre par capture électronique et/ou transitions bêta plus vers plusieurs niveaux de l yttrium, y compris le niveau isomérique et le niveau fondamental. 2 Nuclear Data T 1/2 ( Zr ) : 78,42 (13) h T 1/2 ( m Y ) : 15,84 (18) s Q ( Zr ) : 2832,8 (28) kev 2.1 Electron Capture Transitions Probability (%) Nature lg ft P K P L P M ɛ 0,5 211 (3) 0,745 (10) allowed 6,18 0,8575 (17) 0,1165 (13) 0,0223 (5) ɛ 0,4 266 (3) 0,106 (5) allowed 7,25 0,8615 (16) 0,1134 (13) 0,0216 (5) ɛ 0,3 303 (3) 0,074 (5) allowed 7,52 0,8632 (16) 0,1120 (13) 0,0213 (4) ɛ 0, (3) 0,123 (4) unique 1st forbidden 9,09 0,8677 (15) 0,1082 (12) 0,0208 (4) ɛ 0, (3) 76,2 (3) allowed 6,152 0,8731 (15) 0,1041 (12) 0,0196 (4) 2.2 β Transitions Probability (%) Nature lg ft β 0,1 902 (3) 22,8 (3) allowed 6,152 Surrey Univ. / A.L. Nichols 1 26/05/ /10/2014
2 2.3 Gamma Transitions and Internal Conversion Coefficients P γce α K α L α M α T α π Multipolarity (%) (10 3 ) (10 4 ) (10 4 ) (10 3 ) (10 4 ) γ 1,0(Y) 908,97 (3) 99,873 (23) M4 7,43 (11) 9,06 (13) 1,561 (22) 8,51 (12) γ 3,1(Y) 1620,83 (20) 0,074 (5) M1E2 γ 4,1(Y) 1657,58 (15) 0,106 (5) M1E2 γ 5,1(Y) 1713,1 (3) 0,745 (10) M1E2 γ 2,0(Y) 1744,74 (18) 0,1231 (40) E2 0,1722 (25) 0,186 (3) 0,0317 (5) 0,382 (6) 1,88 (3) 3 Atomic Data 3.1 Y ω K : 0,716 (4) ω L : 0,02 (7) n KL : 1,081 (4) X Radiations Relative probability X K Kα 2 14, ,1 Kα 1 14, Kβ 3 16,7259 Kβ 1 16, ,1 Kβ 5 16,88 Kβ 2 17,0156 3,48 Kβ 4 17,0362 L Ll 1,686 Lα 1,92-1,923 Lη 1,762 Lβ 1,996-2,078 Lγ 2,153-2,347 Surrey Univ. / A.L. Nichols 2 26/05/ /10/2014
3 3.1.2 Auger Electrons Relative probability Auger K KLL 12,205-12, KLX 14,238-14,956 37,6 KXY 16,251-17,034 3,53 Auger L 1,27-1, Electron and Positron Emissions Electrons (per 100 disint.) e AL (Y) 1,27-1, 79,5 (7) e AK (Y) KLL 12,205-12,784 KLX 14,238-14,956 KXY 16,251-17,034 19,4 (3) ec 1,0 T (Y) 1,93-908,97 0,84 (3) ec 1,0 K (Y) 1,93 (3) 0,73 (3) ec 1,0 L (Y) 906,60-906, 0,0 (3) ec 1,0 M (Y) 908,58-908,97 0,017 (1) β 0,1 max: 902 (3) avg: 395,7 (14) 22,8 (3) 5 Photon Emissions 5.1 X-Ray Emissions Photons (per 100 disint.) XL (Y) 1,686-2,347 2,36 (5) XKα 2 (Y) 14, ,08 (13) Kα XKα 1 (Y) 14, ,01 (20) XKβ 3 (Y) 16,7259 XKβ 1 (Y) 16,7381 6,78 (8) K β 1 XKβ 5 (Y) 16,88 XKβ 2 (Y) 17,0156 0,94 (4) K β XKβ 4 (Y) 17, Surrey Univ. / A.L. Nichols 3 26/05/ /10/2014
4 5.2 Gamma Emissions Photons (per 100 disint.) γ ± ,6 (6) γ 1,0 (Y) 908,97 (3) 99,03 (2) γ 3,1 (Y) 1620,81 (20) 0,074 (5) γ 4,1 (Y) 1657,56 (15) 0,106 (5) γ 5,1 (Y) 1713,1 (3) 0,745 (10) γ 2,0 (Y) 1744,72 (18) 0,123 (4) 6 Main Production Modes { Y (p,n)zr Possible impurities: Zr 88(EC)Y 88, Zr m Y (d,2n)zr Y (α,p3n)zr { Zr 90(n,2n)Zr Possible impurities: Zr m Zr 90(p,2n)Nb (EC)Zr Zr 90(p,pn)Zr Zr 90(γ,n)Zr 7 References - R. Sagane, S. Kojima, G. Miyamoto, M. Ikawa. Phys. Rev. 54 (1938) L.A. DuBridge, J. Marshall. Phys. Rev. 58 (1940) 7 (Zr- and Zr-m half-lives) - R. Sagane, S. Kojima, G. Miyamoto, M. Ikawa. Phys. Rev. 57 (1940) M. Goldhaber, E. der Mateosian, G. Scharff-Goldhaber, A.W. Sunyar, M. Deutsch, N.S. Wall. Phys. Rev. 83 (1951) 985 (Half-life, EC decay) - E.K. Hyde, G.D. O Kelley. Phys. Rev. 82 (1951) 944 (Half-life, Gamma-ray emission probabilities) - K. Shure, M. Deutsch. Phys. Rev. 82 (1951) F.J. Shore, W.L. Bendel, R.A. Becker. Phys. Rev. 83 (1951) 688 (Zr-m half-life) - L. Katz, R.G. Baker, R. Montalbetti. Can. J. Phys. 31 (1953) 250 (Zr- and Zr-m half-lives) - F.J. Shore, W.L. Bendel, H.N. Brown, R.A. Becker. Phys. Rev. 91 (1953) 1203 (Zr- and Zr-m half-lives, P(909-keV gamma ray)/p(positron) ratio) - C.P. Swann, F.R. Metzger. Phys. Rev. 100 (1955) M.I. Kuznetsova, V.N. Mekhedov. Izv. Akad. Nauk SSSR, Ser. Fiz. 21 (1957) 1020 (K-capture) - J.H. Hamilton, L.M. Langer, W.G. Smith. Phys. Rev. 119 (1960) 772 Surrey Univ. / A.L. Nichols 4 26/05/ /10/2014
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7 LNE-LNHB/CEA - Table de Radionucléides Zr Emission intensities per 100 disintegrations 0 Zr /2 ; 0 78,42 (13) h 0,21 ps 0,08 ps ,745 0,106 0,074 9/2 ; 2622,1 11/2 ; 2566,55 7/2 ; 2529,8 0,745 0,106 0,074 0,62 ps 2 0,123-5/2 ; 1744,74 0,123 15,84 s ,0 9/2 ; 908,97 76,2 22,8 Stable 0 Y Q = 2832,8 kev % % = 100-1/2 ; 0 Surrey Univ. / A.L. Nichols Scheme page : 1/1 26/05/ /09/2014
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