Advanced operation schemes: two-color, split & delay

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Advanced operation schemes: two-color, split & delay Production of two FEL pulses of different wavelengths with a controllable temporal delay (and) Splitting the FEL pulse into two sequential pulses at SASE3

2 Outline Why do we need two color pulses? How can we produce and deliver them X-ray split and delay device Combination of the both Other schemes under study

3 Baseline SASE3 operation SASE3 undulator (21 segments) Experiment K electron beam SASE λ SASE3 undulator tuned to radiate at wavelength λ Single SASE pulse is transported to the SQS/SCS instrument

4 Two-color SASE3 operation SASE3 undulator (21 segments) + magnetic chicane K1 Magnetic Chicane K2 Experiment electron beam SASE variable delay SASE delay λ 2 > λ 1 Magnetic chicane = electron beam delay Electron beam is delayed in the magnetic chicane Delay can be chosen by tuning the magnetic field (up to ps with sub-fs precision) U2 radiation comes always after (e-beam is delayed only) If wavelengths differ significantly, shorter wavelength goes first (preferably). [1] G. Geloni, et al, Scheme for femtosecond-resolution pump probe experiments at XFELs with two-color ten GW-level X-ray pulses, arxiv:1001.3510 [2] T. Hara et al. Two-colour hard X-ray free-electron laser with wide tunability, doi:10.1038/ncomms3919. [3] A. A. Lutman et al. Experimental Demonstration of Femtosecond Two-Color X-Ray Free-Electron Lasers, doi:10.1103/physrevlett.110.134801.

5 Two-color SASE3 operation SASE3 undulator (21 segments) + magnetic chicane + optical delay Experiment K1 Optical delay K2 electron beam SASE relative delay SASE delay λ 1 < λ 2 Magnetic chicane + mirror chicane = arbitrary delay Electron beam is delayed in the magnetic chicane Photon beam gets delayed in the optical chicane Keep the mirrors fixed, tune using the magnetic chicane

6 Case study for SQS at 630/250 ev SASE3 undulator (21 segments) + magnetic chicane + optical delay 2 off 630eV 7 off 5 active segments 250eV 7 active segments Baseline 20pC e-beam after SASE1 Here we optimized for short pulses mm

7 First undulator (second pulse) 630 ev Mean Energy/pulse: 5e-5 J Mean #ph/pulse : 5e11 0.5 μm fwhm (1.5 fs) 50 μj 50 GW

8 Second undulator (first pulse) 250 ev Mean Energy/pulse: 7e-5 J Mean #ph/pulse : 1.75e12 1 μm fwhm (3 fs) 70 μj 30 GW

9 Two sources problem 630 ev 1.8e18 ph/cm 2 Two sources and one focusing system -> two images Two mirrors -> only one image without aberrations We can tune both KB mirrors to image the intermediate spot in both planes 250 ev 4.5e18 ph/cm 2 I1.5 Both KBs focused at S1.5 630 ev Interm. 250 ev S1 S1.5 S2

10 Concept of optical X-ray split and delay device (XBSD) for SASE3 (by AlexanderYaroslavtsev) Located upstream of both instruments M Separated asymmetric paths Two mirror coatings: B4C (up to 1500 ev) Ni or Ru (up to 3000 ev) Plane mirrors -> does not affect focusing M

Recombine any two Advanced operation schemes: two-color, split & delay Svitozar Serkez (on behalf of WP72, SCS, SQS) 24.01.2017 11 Concept of optical X-ray split and delay device (XBSD) for SASE3 (by AlexanderYaroslavtsev) Upgradeable with zero-order mirror (ZOM) G Recombination of different grating reflection orders at optical axis possible 0 th odrer λ 1 0 th odrers Grating Grating 1 st odrer λ 2 (mono) 1 st odrer λ 1 (mono) 1 st odrer λ 1 (mono) λ 1 pink beam λ 2 λ 1

12 Two-color SASE + XBSD combination λ x == λ x (sase) (by AlexanderYaroslavtsev) Undulator mode XBSD mode Result N. of pulses N. of frequencies (boring) mono λ 1 (mono) Δt (fs ps) λ 1 (mono) 2 1 mono λ 1 mono + ZOM 0 th λ 1 Δt (fs ps) λ 1 (mono) 2 1 sase/mono pink λ 1 Δt (fs ps) λ 1 2 2 sase mono XFEL baseline λ 1 (mono) Δt 1 (fs) λ 1 (mono) Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 mono λ 1 Δt 1 (fs) λ 1 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 sase/mono pink λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 1 4 1 sase mono + ZOM 1 st λ 1 (mono) Δt 2 (fs ps) λ 2 (mono) 2 2 mono λ 1 Δt 1 (fs) λ 2 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 2 (mono) 3 2 sase/mono pink λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 2 4 2 sase λ 1

13 Two-color SASE + XBSD combination λ x == λ x (sase) (by AlexanderYaroslavtsev) Undulator mode XBSD mode Result N. of pulses N. of frequencies mono λ 1 (mono) Δt (fs ps) λ 1 (mono) 2 1 mono XBCD scheme λ 1 mono + ZOM 0 th λ 1 Δt (fs ps) λ 1 (mono) 2 1 sase/mono pink λ 1 Δt (fs ps) λ 1 2 2 sase mono λ 1 (mono) Δt 1 (fs) λ 1 (mono) Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 mono λ 1 Δt 1 (fs) λ 1 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 sase/mono pink λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 1 4 1 sase mono + ZOM 1 st λ 1 (mono) Δt 2 (fs ps) λ 2 (mono) 2 2 mono λ 1 Δt 1 (fs) λ 2 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 2 (mono) 3 2 sase/mono pink Two-color scheme interference terms λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 2 4 2 sase Δt 1 (fs) λ 2 λ 1

14 Two-color SASE + XBSD combination λ x == λ x (sase) (by AlexanderYaroslavtsev) Undulator mode XBSD mode Result N. of pulses N. of frequencies mono λ 1 (mono) Δt (fs ps) λ 1 (mono) 2 1 mono λ 1 mono + ZOM 0 th λ 1 Δt (fs ps) λ 1 (mono) 2 1 sase/mono pink λ 1 Δt (fs ps) λ 1 2 2 sase mono λ 1 (mono) Δt 1 (fs) λ 1 (mono) Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 XBCD 1 mono scheme λ 1 Δt 1 (fs) λ 1 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 sase/mono pink λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 1 4 1 sase mono + ZOM 1 st λ 1 (mono) Δt 2 (fs ps) λ 2 (mono) 2 2 mono λ 1 Δt 1 (fs) λ 2 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 2 (mono) 3 2 sase/mono interference terms pink λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 2 4 2 sase λ 1 λ 1 λ 1 Δt 2 (fs ps)

15 Two-color SASE + XBSD combination λ x == λ x (sase) (by AlexanderYaroslavtsev) Undulator mode XBSD mode Result N. of pulses N. of frequencies mono λ 1 (mono) Δt (fs ps) λ 1 (mono) 2 1 mono λ 1 mono + ZOM 0 th λ 1 Δt (fs ps) λ 1 (mono) 2 1 sase/mono pink λ 1 Δt (fs ps) λ 1 Interference 2 2 sase terms mono λ 1 (mono) Δt 1 (fs) λ 1 (mono) Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 mono λ 1 Δt 1 (fs) λ 1 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 sase/mono pink λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 1 4 1 sase mono + ZOM 1 st λ 1 (mono) Δt 2 (fs ps) λ 2 (mono) 2 2 mono λ 1 Δt 1 (fs) λ 2 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 2 (mono) 3 2 sase/mono pink λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 2 4 2 sase Δt 1 (fs) λ 2 λ 1 λ 2 λ 1 λ 2 λ 1 Δt 2 (fs ps)

16 Coherent Anti-Stokes Raman Scattering (CARS) Correlation Spectroscopy Undulator mode XBSD mode Result N. of pulses N. of frequencies mono λ 1 (mono) Δt (fs ps) λ 1 (mono) 2 1 mono λ 1 mono + ZOM 0 th λ 1 Δt (fs ps) λ 1 (mono) 2 1 sase/mono pink λ 1 Δt (fs ps) λ 1 2 2 sase mono λ 1 (mono) Δt 1 (fs) λ 1 (mono) Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 mono λ 1 Δt 1 (fs) λ 1 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 (mono) Δt 1 (fs) λ 1 (mono) 4 1 sase/mono pink λ 1 Δt 1 (fs) λ 1 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 1 4 1 sase mono + ZOM 1 st λ 1 (mono) Δt 2 (fs ps) λ 2 (mono) 2 2 mono λ 1 Δt 1 (fs) λ 2 mono + ZOM 0 th λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 2 (mono) 3 2 sase/mono pink λ 1 Δt 1 (fs) λ 2 Δt 2 (fs ps) λ 1 Δt 1 (fs) λ 2 4 2 sase Δt 2 λ 2 λ 1 λ 2 (mono) λ 1

Wavelength Advanced operation schemes: two-color, split & delay Svitozar Serkez (on behalf of WP72, SCS, SQS) 24.01.2017 17 Coherent Anti-Stokes Raman Scattering (CARS) Correlation Spectroscopy λ 2 0 th odrers (2 pulses) Grating 1 st odrer λ 1 (mono) λ 1 (mono) λ 1 1 st odrer λ 2 (mono) Δt 2 λ 2 λ 1 Time Δt 2 sample Δt 1 =0 λ 1 λ 2 λ 1 (mono) λ 1 λ 2 Two pulses of different wavelengths are generated in the undulator Grating is tuned to monochromatize one of the pulses in 1 st order reflection 0 th order reflection carries both SASE pulses and is recombined with ZOM Monochromatic pulse is delayed in XBSD by Δt 2 Story continues in talk by Justine Schlappa later today ω 1 ω 1 ω 2 Δt 2 ω out δω Ω

delay, ps Advanced operation schemes: two-color, split & delay Svitozar Serkez (on behalf of WP72, SCS, SQS) 24.01.2017 18 Comparison of delay ranges Two-color scheme: XBSD: λ 2 > λ 1 optical delay out: depends on electron beam energy up to (0 1 ps) depends on photon energy, estimated (-7 7 ps) up to 4 ps per single scan 8 6 optical delay in: estimated (-100 100 fs) 4 2 0-2 -4-6 -8 0 20 40 60 80 100 stage position z, mm Example of the delay ranges 1000 ev, 5 fs pulse

19 Other schemes Circular polarizarion at SASE3 see S.Serkez, et al., Circular polarization opportunities at the SASE3 undulator line of the European XFEL, arxiv:1608.08175 Self-seeding see S.Serkez, Design and Optimization of the Grating Monochromator for Soft X-Ray Self-Seeding FELs, doi:10.3204/desy-thesis-2015-043 Ongoing R&D on attosecond pulse generation

20 End words Two-color scheme: robust, easy to set-up same pulse duration tunable delay, scan possible large max. range, up to 2500 250 ev, independent scan possible for both wavelengths XBSD: introduces tunable delay, scan possible does not affect baseline focusing can create two identical pulses allows delivery of SASE and monochromatic pulses with a given delay (with ZOM) Combination of the two: gives large added values, see Table Other schemes are under active study If you are interested please let us know

21 Thank you WP72, SCS, SQS, WP78, MPY(DESY)