Distribution Characteristics of Polycyclic Aromatic Hydrocarbons and Black Carbon in Road Dusts from Typical Cities of China and India
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1 ENVIRONMENTAL SCIENCE Vol 33 No 4 Apr PAHs BC ~ GC-MS PAHs 2 30 ~ 22 2 μg g - 1 b ghi PAHs 4 85 ~ 30 5 μg g PAHs BC 2 PAHs BC PAHs X53 A Distribution Characteristics of Polycyclic Aromatic Hydrocarbons and Black Carbon in Road Dusts from Typical Cities of China and India PAN Su-hong ZHANG Gan 2 SUN Ya-li 3 XIE Qi-lai College of Natural Resources and Environment South China Agricultural University Guangzhou China 2 State Key Laboratory of Organic Geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou China 3 State Key Laboratory of Isotope Geochemistry Guangzhou Institute of Geochemistry Guangzhou China 4 Key Laboratory of Soil Environment and Waste Reuse in Agriculture of Guangdong High Education Institutions Guangzhou China Abstract In order to investigate the distribution characteristics of polycyclic aromatic hydrocarbons PAHs and black carbon BC in road dusts in typical cities of Beijing Shanghai Guangzhou and Wuhan in China and Kolcata in India samples were collected in urban roads during Dec 2007 to Feb 2009 The total 16 PAHs concentrations in metro cities from China were μg g - 1 which was dominated by FLA PHE PYR CHR BBF and BGP PAHs contents were in the range of μg g - 1 in Kolcata from India which was dominated by NAP Higher levels of BC in Chinese cities than India city were likely due to different power structures and consumes The correlation between PAHs and BC showed different characteristics in different city which might be reflected diverse sources Diagnostic ratios demonstrated that the main source of PAHs was from the emission of vehicle and coal combustion is another possible source Key words China India road dust polycyclic aromatic hydrocarbons PAHs black carbon BC 3 2 PAHs BC BC ~ pansuhong0120@ 163 com
2 ~ μg g - 1 PAHs PAHs 13 PAHs BC PAHs ~ PAHs PAHs GDP PAHs 10 m 2 16 PAHs 1 2 EPA PAHs PAHsNAP ACE ACEY FLU PHE ANT FLA PYR a BAA CHY b BBF k BKF a BAP cd INP a h DIB ghi BGP 50% PAHs 5 -d8 -d10 d10 -d10 -d12 GC-MS 64% ± 21% 79% ± 18% 92% ± 11% 113% ± 25% 101% ± 33% NAP 2 3 BC 6 10 mg HCl h Elementar Vario EL Ⅲ PAHs PAHs PAHs 1 PAHs 2 30 ~ 22 2 μg g ~ 22 2 μg g PAHs 0 82 ~ 10 6 μg g PAHs 3 44 ~ 6 85 μg g FLA PHE PYR CHR BBF BGP PAHs 59% ~ 69% 2 NAP PAHs PAHs ~ 32 6 μg g dusts from different cities PAHs 11 PAHs 4 85 ~ 1 Fig 1 PAHs Relative distributions of PAHs in road
3 Table 1 1 PAHs BC 1 Concentrations of PAHs and BC in road dusts around the world N Σ PAH /μg g - 1 BC /mg g ~ ± ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ ~ PAHs PAHs BC PAHs PAHs BC BC BC PAHs 21 PAHs BC n = 49 P > 0 05 PAHs PAHs BC PAHs BC PAHs n = 13 r 2 = 0 77 P < 0 05 P > 0 19 PAHs PAHs BC BC PAHs 2 2 BC BC BC 1 BC 5 46 ~ 27 7 mg g PAHs 7 BC PAHs - BC BC BC 2 PAHs BC 22 BC BC ~ 9 22 mg g - 1 PAHs BC BC 11 BC 20
4 PAHs BC 0 28 ~ ~ ~ PAHs 0 17 ~ ~ ~ ~ BAA /CHR BAP /BGP INP /BGP PAHs PAHs PAHs 0 44 ~ ~ ~ PAHs 0 52 ~ ~ ~ ~ ~ ~ PAHs 0 49 ~ ~ ~ 1 04 PAHs 0 52 ~ ~ ~ 1 08 PAHs LMW 3 PAHs HMW 4 PAHs LMW /HMW > 1 < 1 27 / + ANT / < 0 1 PAHs > NAP 3 LMW /HMW > 1 ANT /178 1 PAHs 2 Fig 2 ANE /178 LMW /HMW Plot of ANE /178 ratios against LMW /HMW ratios in road dusts BAA /CHR BAP /BGP INP /BGP PAHs BAP /BGP Paromita Chakraborty PAHs PAHs 1 Guo Z G Lin T Zhang G et al Occurrence and sources of polycyclic aromatic hydrocarbons and n-alkanes in PM2 5 in the Table 2 2 PAHs Diagnostic ratios of PAHs in road dusts FLA PHE PYR CHR BBF BGP PAHs 2 NAP PAHs BC 2 PAHs BC PAHs BC PAHs BC 3 PAHs
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