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- Εἰλείθυια Βασιλόπουλος
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1 ... - M.abdollahpour@yahoo.com () ( ) - (// // )..... /.. ph :.[]...[-] [].. 1 HOBr 2 Ozonation Process 64
2 ( H 2 O) 5 AlOH Br (H 2O) 4 AlOHBr () + ( H2O) 4 Al(OH) 2 + Br (H 2O) 3Al(OH) 2 Br () / /.[] / / /.. / /.[] / /... ph... 2 Design-Expert 3 Response Surface Method (RSM). ) (..[-]. (IPFs).[ ] ph.[ ] IPF.[ ]. ph.[-] ( H 2O) 6 Al + Br (H 2O) 5 AlBr () 1 U.S. Environmental Protection Agency (USEPA) 65
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3 ....[ ] --...[]. ( ). ( 2 ) /...[]... () ( ). 4 Box-Behnken 5 Central Composite 6 Central Composite Design (CCD) ( )... [] -. 1 Contour 2 Curvature 3 Center Point 66
4 ... () - - () - - +/=β+ + - ( 3 )-/=-β / / / / / X 1 ( ) / / X 2 ( ) / / / / / X 3 ph. ph ph. - / (R 2 ) 3 Settling Time 4 Bench meter/180mi 5 MARTINI instruments 6 Advanced compact/i.c R-squared --. /.. / 1 Deionized Water 2 Merck 67
5 ... ) ( / / / / / / / / / / / / / / / / / / / / ph - ( ) ( ) X 3 X 2 X 1 / / / / / / / / / / - - / / - / / - / / / / -/ / / -/ / / / -/ / / / -/ / / -/ / / -/ / / / / / / / / / / / / /. / ph ph / ph -. X 2 X 1. () Y = X X X X 1 X X 1 X X 3 X 2-37X X 2... (/ ) ph 68
6 .... / ph.. / ph ph. ph / ph. ph.. ( ) ( ) ( ) - ph ph - - ( ) ph ph - ph -. ph / ph ph ph. / 69
7 ... ph ph / ph / / ph. - ph. / / ph ph.. / / ph / /.. /... ph ph ph ph / ph. / ph / ph. ph. 70
8 Zhang, Y.J., Zhou, L.L., Zeng, G., Song Z.G., and Li, G.B. (2010). Factors affecting the formation of trihalomethanes in the presence of bromide during chloramination. J. of Appl. Phys. and Eng., 11(8), Rizzo, L., Belgiomo, V., and Gallo, M.S. (2005). Removal of THM precursors from a high-alkaline surface water by enhanced coagulation and behavior of THMFP toxicity. J. of Desalination, 176, Echigo, S., Itoh, S., and Kuwahara, M. (2007). Bromide removal by hydrotalcite-like compounds in a continuous system. J. of Water Science and Technology, 56, Camel, V., and Bermond, A. (1998). The use of ozone and associated oxidation processes in drinking water treatment. J. of Water Research, 32(11), Shukairy, H.M., Miltner, R.J., and Summers, R.S. (1995). Bromide s effect on DBP formation, speciation, and control, part 2, Biotreatment. J. of Water Wks. Assoc., 87(10), Liu, S., Zhu, Z., Qiu, Y., and Zhao, J. (2011). Effect of ferric and bromide ions on the formation and speciation of disinfection byproducts during chlorination. J. of Environmental Sciences, 23(5), US. Environmental Protection Agency (USEPA). (1998). Disinfectants and disinfectants by-products: final rule, Federal Register, 63(24), WHO. (1990). IARC monographs on the evaluation of carcinogenic risks to humans, World Health Organization, Geneva. 9. Watson, K., Farré, M.J., and Knight, N. (2012). Review strategies for the removal of halides from drinking water sources, and their applicability in disinfection by-product minimization. J. of Environmental Management, 110, Shi, B., Li, G., Wang, D., Feng, C., and Tang, H. (2007). Removal of direct dyes by coagulation: The performance of preformed polymeric aluminum species. J. of Hazard. Mater., 143, Wang, D., Sun, W., Xu, Y., Tang, H., and Gregory, J. (2004). Speciation stability of inorganic polymer flocculant-pacl. J. of Colloids Surf. A: Physicochem. Eng. Aspects, 243, Jiang, J. Q. (2001). Development of coagulation theory and prepolymerized coagulants for water Treatment. J. of Separation and Purification Methods, 30, Ye, C., Wang, D., Shi, B., Yu, J., Qu, J., Edwards, M., and Tang, H. (2007). Alkalinity effect of Coagulation with polyaluminum chlorides: Role of electrostatic patch. J. of Colloids Surf. A: Physicochem. Eng. Aspects, 294, Ge, F., Shu, H., and Dai, Y. (2007). Removal of bromide by aluminum chloride coagulant in the presence of humic acid. J. of Hazard. Mater., 147, Gunten, U.V. (2003). Review ozonation of drinking water Part II disinfection and by-product formation in presence of bromide, iodide or chlorine. J. of Water Research, 37, Omelia, C.R., and Shin, J.Y. (2001). Removal of particle using dual media filtration modeling and experimental studies. J. of Water Supply, IWA., 1(4),
9 Eric, H., and Kara, H. (2002). Optimizing coagulant conditions for the Worcester water filtration plants, A Major Qualifying Project Report Submitted to the Faculty of Worcester Polytechnic Institute, USA. 18. Malhutra, S. (1994). Polyaluminum chloride as an alternative coagulant. Proc. 20 th WEDC Conference Colombo, Sri Lanka. 19. Tang, H.X., and Luan, Z.K. (1995). Features and mechanism for coagulation flocculation process of polyaluminum chloride. J. of Environ. Sci., 7(2), Luan, Z.K. (1997). Theory and application of inorganic polymer flocculant-polyaluminium chloride. Doctoral Dissertation, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing. 21. Liu, W., Huang, H., and Peng, J. (2001). Application of polyaluminum chloride in Shenzhen water supply, Qingyouan Water Purification Water Supply Group Ltd., Shenzhen, China. 22. Ge, F., and Zhu, L., (2008). Effects of coexisting anions on removal of bromide in drinking water by coagulation. J. of Hazard. Mater., 151, Piepel, G., Anderson, C.M., and Redgate, P.E. (1993). Response surface designs for irregularly-shaped regions. Proc. of the Section on Physical and Engineering Sciences, American Statistical Association, Alexandria, Virginia, Aslan, N., and Cebeci, Y. (2007). Application of box-behnken design and response surface methodology for modeling of some Turkish coals. J. of Fuel, 86,
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