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1 Decay Scheme Zr- (half-life of 78.42 h) undergoes 100% EC/positron decay (Q EC of 2832.8(28) kev) to various nuclear levels, including the metastable and ground states of Y-. Le zirconium se désintègre par capture électronique et/ou transitions bêta plus vers plusieurs niveaux de l yttrium, y compris le niveau isomérique et le niveau fondamental. 2 Nuclear Data T 1/2 ( Zr ) : 78,42 (13) h T 1/2 ( m Y ) : 15,84 (18) s Q ( Zr ) : 2832,8 (28) kev 2.1 Electron Capture Transitions Probability (%) Nature lg ft P K P L P M ɛ 0,5 211 (3) 0,745 (10) allowed 6,18 0,8575 (17) 0,1165 (13) 0,0223 (5) ɛ 0,4 266 (3) 0,106 (5) allowed 7,25 0,8615 (16) 0,1134 (13) 0,0216 (5) ɛ 0,3 303 (3) 0,074 (5) allowed 7,52 0,8632 (16) 0,1120 (13) 0,0213 (4) ɛ 0,2 1088 (3) 0,123 (4) unique 1st forbidden 9,09 0,8677 (15) 0,1082 (12) 0,0208 (4) ɛ 0,1 1924 (3) 76,2 (3) allowed 6,152 0,8731 (15) 0,1041 (12) 0,0196 (4) 2.2 β Transitions Probability (%) Nature lg ft β 0,1 902 (3) 22,8 (3) allowed 6,152 Surrey Univ. / A.L. Nichols 1 26/05/2014 16/10/2014

2.3 Gamma Transitions and Internal Conversion Coefficients P γce α K α L α M α T α π Multipolarity (%) (10 3 ) (10 4 ) (10 4 ) (10 3 ) (10 4 ) γ 1,0(Y) 908,97 (3) 99,873 (23) M4 7,43 (11) 9,06 (13) 1,561 (22) 8,51 (12) γ 3,1(Y) 1620,83 (20) 0,074 (5) M1E2 γ 4,1(Y) 1657,58 (15) 0,106 (5) M1E2 γ 5,1(Y) 1713,1 (3) 0,745 (10) M1E2 γ 2,0(Y) 1744,74 (18) 0,1231 (40) E2 0,1722 (25) 0,186 (3) 0,0317 (5) 0,382 (6) 1,88 (3) 3 Atomic Data 3.1 Y ω K : 0,716 (4) ω L : 0,02 (7) n KL : 1,081 (4) 3.1.1 X Radiations Relative probability X K Kα 2 14,8829 52,1 Kα 1 14,9585 100 Kβ 3 16,7259 Kβ 1 16,7381 25,1 Kβ 5 16,88 Kβ 2 17,0156 3,48 Kβ 4 17,0362 L Ll 1,686 Lα 1,92-1,923 Lη 1,762 Lβ 1,996-2,078 Lγ 2,153-2,347 Surrey Univ. / A.L. Nichols 2 26/05/2014 16/10/2014

3.1.2 Auger Electrons Relative probability Auger K KLL 12,205-12,784 100 KLX 14,238-14,956 37,6 KXY 16,251-17,034 3,53 Auger L 1,27-1, 579 4 Electron and Positron Emissions Electrons (per 100 disint.) e AL (Y) 1,27-1, 79,5 (7) e AK (Y) KLL 12,205-12,784 KLX 14,238-14,956 KXY 16,251-17,034 19,4 (3) ec 1,0 T (Y) 1,93-908,97 0,84 (3) ec 1,0 K (Y) 1,93 (3) 0,73 (3) ec 1,0 L (Y) 906,60-906, 0,0 (3) ec 1,0 M (Y) 908,58-908,97 0,017 (1) β 0,1 max: 902 (3) avg: 395,7 (14) 22,8 (3) 5 Photon Emissions 5.1 X-Ray Emissions Photons (per 100 disint.) XL (Y) 1,686-2,347 2,36 (5) XKα 2 (Y) 14,8829 14,08 (13) Kα XKα 1 (Y) 14,9585 27,01 (20) XKβ 3 (Y) 16,7259 XKβ 1 (Y) 16,7381 6,78 (8) K β 1 XKβ 5 (Y) 16,88 XKβ 2 (Y) 17,0156 0,94 (4) K β XKβ 4 (Y) 17,0362 2 Surrey Univ. / A.L. Nichols 3 26/05/2014 16/10/2014

5.2 Gamma Emissions Photons (per 100 disint.) γ ± 511 45,6 (6) γ 1,0 (Y) 908,97 (3) 99,03 (2) γ 3,1 (Y) 1620,81 (20) 0,074 (5) γ 4,1 (Y) 1657,56 (15) 0,106 (5) γ 5,1 (Y) 1713,1 (3) 0,745 (10) γ 2,0 (Y) 1744,72 (18) 0,123 (4) 6 Main Production Modes { Y (p,n)zr Possible impurities: Zr 88(EC)Y 88, Zr m Y (d,2n)zr Y (α,p3n)zr { Zr 90(n,2n)Zr Possible impurities: Zr m Zr 90(p,2n)Nb (EC)Zr Zr 90(p,pn)Zr Zr 90(γ,n)Zr 7 References - R. Sagane, S. Kojima, G. Miyamoto, M. Ikawa. Phys. Rev. 54 (1938) 542 - L.A. DuBridge, J. Marshall. Phys. Rev. 58 (1940) 7 (Zr- and Zr-m half-lives) - R. Sagane, S. Kojima, G. Miyamoto, M. Ikawa. Phys. Rev. 57 (1940) 1179 - M. Goldhaber, E. der Mateosian, G. Scharff-Goldhaber, A.W. Sunyar, M. Deutsch, N.S. Wall. Phys. Rev. 83 (1951) 985 (Half-life, EC decay) - E.K. Hyde, G.D. O Kelley. Phys. Rev. 82 (1951) 944 (Half-life, Gamma-ray emission probabilities) - K. Shure, M. Deutsch. Phys. Rev. 82 (1951) 122 - F.J. Shore, W.L. Bendel, R.A. Becker. Phys. Rev. 83 (1951) 688 (Zr-m half-life) - L. Katz, R.G. Baker, R. Montalbetti. Can. J. Phys. 31 (1953) 250 (Zr- and Zr-m half-lives) - F.J. Shore, W.L. Bendel, H.N. Brown, R.A. Becker. Phys. Rev. 91 (1953) 1203 (Zr- and Zr-m half-lives, P(909-keV gamma ray)/p(positron) ratio) - C.P. Swann, F.R. Metzger. Phys. Rev. 100 (1955) 1329 - M.I. Kuznetsova, V.N. Mekhedov. Izv. Akad. Nauk SSSR, Ser. Fiz. 21 (1957) 1020 (K-capture) - J.H. Hamilton, L.M. Langer, W.G. Smith. Phys. Rev. 119 (1960) 772 Surrey Univ. / A.L. Nichols 4 26/05/2014 16/10/2014

- S. Monaro, G.B. Vingiani, R. van Lieshout. Physica 27 (1961) 985 (Half-life, Gamma-ray energies and emission probabilities, EC/positron ratio) - L.A. Rayburn. Phys. Rev. 122 (1961) 168 - D.A. Howe, L.M. Langer, D. Wortman. Nucl. Phys. 37 (1962) 476 (Gamma-ray emissions feeding 909-keV level) - E.T. Bramlitt, R.W. Fink. J. Inorg. Nucl. Chem. 24 (1962) 1321 (Y-m half-life) - Y. Awaya, Y. Tendow. J. Phys. Soc. Japan 19 (1964) 606 (1700(100)-keV gamma ray) - D.M. van Patter, S.M. Shafroth. Nucl. Phys. 50 (1964) 113 (Zr- and Zr-m half-lives, Gamma-ray energies and emission probabilities, EC energies and transition probabilities, EC/positron ratio) - S.A. Durrani, W. Köhler. Trans. Am. Nucl. Soc. 9 (1966) 479 (Y-m half-life) - H.P. Yule. Nucl. Phys. A94 (1967) 442 (Y-m half-life) - P. Bornemisza-Pauspertl, P. Hille. Osterr. Akad. Wiss. Math-Naturw. Kl. Sitzber. Abt. II 176 (1968) 227 (Y-m half-life) - J.E. Draper, J.A. McCray. Nucl. Phys. A120 (1968) 234 (Zr- and Zr-m half-lives, Gamma-ray energies and emission probabilities) - P.F. Hinrichsen, S.M. Shafroth, D.M. van Patter. Phys. Rev. 172 (1968) 1134 (Y- nuclear levels) - P.F. Hinrichsen. Nucl. Phys. A118 (1968) 538 (Gamma-ray energies and emission probabilities, EC transition probabilities, Positron emission probability, P(909- kev gamma ray)/p(511-kev gamma ray) ratio) - R. Gunnink, J.B. Niday, R.P. Anderson, R.A. Meyer. Lawrence Radiation Laboratory report UCID-15439 (1969) (Gamma-ray energies and emission probabilities) - E.L. Robinson, R.C. Hagenauer, E. Eichler. Nucl. Phys. A123 (1969) 471 (Zr- and Zr-m half-lives, Gamma-ray energies and emission probabilities) - St. Gagneux, P. Huber, H. Leuenberger, P. Nyikos. Helv. Phys. Acta 43 (1970) 39 (Zr- half-life variation) - N.B. Gove, M.J. Martin. Nucl. Data Tables 10 (1971) 205 (EC/positron ratios) - R. Arlt, N.G. Zaitseva, B. Kracik, M.G. Loshchilov, G. Musiol, Chan Thanh Minh, H. Strusny. Bull. Acad. Sci. USSR, Phys. Ser. 35 (1972) 52 (Gamma-ray energies and emission probabilities, EC transition probabilities, Positron emission probability) - H. Leuenberger. Physica 64 (1973) 621 (Theoretical modelling of variation in Zr- half-life) - W. Beens. PhD thesis, Vrije Universiteit, Amsterdam (1973) (Half-lives of Y- nuclear levels) - R.L. Heath. updated 1998, ANCR-1000-2 (1974) (Half-life, Gamma-ray energies and emission probabilities) - F.P. Larkins. At. Data Nucl. Data Tables 20 (1977) 311 (Auger-electron energies) - W. Bambynek, H. Behrens, M.H. Chen, B. Crasemann, M.L. Fitzpatrick, K.W.D. Ledingham, H. Genz, M. Mutterer, R.L. Intemann. Rev. Mod. Phys. 49 (1977) 77 (EC/positron ratio) - W. Bambynek, H. Behrens, M.H. Chen, B. Crasemann, M.L. Fitzpatrick, K.W.D. Ledingham, H. Genz, M. Mutterer, R.L. Intemann. Erratum: Rev. Mod. Phys. 49 (1977) 961 (EC/positron ratio) - A.D. Baillie, K.W.D. Ledingham, J.G. Lynch, M. Campbell. J. Phys. G: Nucl. Phys 5 (1979) 1433 (P(EC)/P(positron), P(KX)/P(909-keV gamma ray) and P(K)/P(positron) ratios, Gamma-ray energies and emission probabilities) - J.J. Hamill, A. Zemel. KVI 1983 Annual Report (1984) 18 ((M1E2) multipolarity of 1713-keV gamma ray) - R.T. Skelton, R.W. Kavanagh. Nucl. Phys. A414 (1984) 234 (Half-life, EC transition probabilities) Surrey Univ. / A.L. Nichols 5 26/05/2014 16/10/2014

- J. Hamill, A.J. Hoeven, J. van Klinken, V.A. Wichers, A. Zemel. KVI 1984 Annual Report (1985) 18 ((M1E2) multipolarity of 1713-keV gamma ray) - L. Funke, G. Winter, J. Döring, L. Käubler, H. Prade, R. Schwengner, E. Will, Ch. Protochristov, W. Andrejtscheff, L.G. Kostova, P.O. Lipas, R. Wirowski. Nucl. Phys. A541 (1992) 241 (Gamma-ray energies and emission probabilities, Half-lives of Y- nuclear levels) - K. Kawade, H. Yamamoto, A. Tanaka, A. Hosoya, T. Katoh, T. Iida. JAERI report JAERI-M-92-027 (1992) 364 (Zr-m half-life) - E. Schönfeld. PTB Report PTB-6.33-95-2 (1995) (P(K), P(L), P(M), P(N), P(O)) - S. Itoh, M. Yasuda, H. Yamamoto, T. Iida, A. Takahashi, K. Kawade. JAERI Report JAERI-Conf-95-008 (1995) 185 (Y-m half-life) - E. Schönfeld, H. Janssen. Nucl. Instrum. Methods Phys. Res. A369 (1996) 527 (Fluorescence yields, X-ray emission probability ratios, Auger-electron emission probability ratios) - S. Lahiri, B. Mukhopadhyay, N.R. Das. Appl. Rad. Isot. 48 (1997) 883 (Y-(alpha,p3n)Zr- mode of production) - E. Schönfeld, G. Rodloff. PTB Report PTB-6.11-98-1 (1998) (Auger electrons) - E. Schönfeld. Appl. Rad. Isot. 49 (1998) 1353 (P(K), P(L), P(M), P(N), P(O)) - E. Schönfeld, G. Rodloff. PTB Report PTB-6.11-1999-1 (1999) (X(K)) - E. Schönfeld, H. Janssen. Appl. Rad. Isot. 52 (2000) 595 (P(X), P(Ae)) - I.M. Band, M.B. Trzhaskovskaya, C.W. Nestor Jr., P.O. Tikkanen, S. Raman. At. Data Nucl. Data Tables 81 (2002) 1 (Theoretical ICC) - S. Raman, C.W. Nestor Jr., A. Ichihara, M.B. Trzhaskovskaya. Phys. Rev. C66 (2002) 044312 (Theoretical ICC) - T. Kibédi, T.W. Burrows, M.B. Trzhaskovskaya, P.M. Davidson, C.W. Nestor Jr. Nucl. Instrum. Methods Phys. Res. A5 (2008) 202 (Theoretical ICC and IPF coefficients) - M. Wang, G. Audi, A.H. Wapstra, F.G. Kondev, M. MacCormick, X. Xu, B. Pfeiffer. Chin. Phys. C36 (2012) 1603 (Q-value) - B. Singh. Nucl. Data Sheets 114 (2013) 1 (Nuclear levels) Surrey Univ. / A.L. Nichols 6 26/05/2014 16/10/2014

LNE-LNHB/CEA - Table de Radionucléides Zr 40 49 Emission intensities per 100 disintegrations 0 Zr 40 49 9/2 ; 0 78,42 (13) h 0,21 ps 0,08 ps 5 4 3 0,745 0,106 0,074 9/2 ; 2622,1 11/2 ; 2566,55 7/2 ; 2529,8 0,745 0,106 0,074 0,62 ps 2 0,123-5/2 ; 1744,74 0,123 15,84 s 1 3 9 9,0 9/2 ; 908,97 76,2 22,8 Stable 0 Y 39 50 Q = 2832,8 kev % % = 100-1/2 ; 0 Surrey Univ. / A.L. Nichols Scheme page : 1/1 26/05/2014-17/09/2014