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1 ,.. 3, : ; ; -., -,, -.,., - -, [1].,, [2],. [2], 1., -,, -,,. - [3]., ( -,..).,,. -., [4],, -,. -,., -,.. - A n+1 A n A [5]. [6] ,,, -. korenchenko@physics.susu.ac.ru 3 -,,, -. sas@physics.susu.ac.ru 4 -,,, brg@fmp.ru 20. «..»
2 ..,..,.., - -,. [1] -,. [7].. [8]. - (n > 50), -.,,,,, -,.,,. - :, -. -., - -,. -, , LAMMPS [9]. ( r) - ( u). ( - ),. -, [10]. r r Cu Ar - - = 0,0123, = 3, [1],,,. -, - - [11]., Ar -. : ,08, , , Ar-Ar., -. y = Cx 2. Cu Cu Cu Ar., [11]: 2014, 6, 4 21
3 CM σ =, 2 u τ N AV M, u,, V. 6, , , [11]. Cu Cu Cu Ar., Cu Cu = 300 = 1500, 10 %., Ar Ar 0,15. -, :, - ( ).,,.,,. -, [11]: P = 1 exp( u tcnσ ), (1) t c, n, -. (. 2),, , - 0,6., - t > t c (.. 2). - :. 2, «..»
4 ..,..,.., y = y + A exp( R T ). (2) , - (y 0 = 23,76, A = 25,28, R 0 = 1, ). -, 15, : -.. 4, ( ) - ( ), 100., Cu Ar. 0,3 / 3., 0, , 25., , -, n < 15 0,01., , 6, 4 23
5 - : 1. - (n < 50),..,.,,,. (2),. 2. N ij, i j, - -, P -,, (1)., P N ij,, ,.. - /..,.. // I. /..,..,..,.. // Becker, R. The kinetic treatment of nuclear formation in supersaturated vapors / R. Becker, W. Doring // Ann. Phys Vol. 24. P Krasnochtchekov, P. Molecular dynamics simulations of cluster nucleation during inert gas condensation / P. Krasnochtchekov, R.S Averback // The Journal of Chemical Physics Vol P Brady, J.W. Cluster dynamics: A classical trajectory study of A + A n? A * n+1 / J.W. Brady, J.D. Doll, D.L. Thompson // The Journal of Chemical Physics Vol. 71, 6. P Insepov, Z.A. The kinetics of condensation behind the shock front / Z.A. Insepov, E.M. Karatajev, G.E. Norman // Zeitschrift fur Physik D Atoms, Molecules and Clusters Vol. 20. P /..,..,..,.. // , 4. C ,.. /..,..,.. // , Plimpton, S. Fast Parallel Algorithms for Short Range Molecular Dynamics / S. Plimpton // Journal of Computational Physics Vol P Kesala, E. Molecular dynamics simulation of pressure dependence of cluster growth in inert gas condensation / E. Kesala, A. Kuronen, K. Nordlund // Physical Review B Vol. 75. P ,.. /....:, «..»
6 ..,..,.. Bulletin of the South Ural State University Series Mathematics. Mechanics. Physics 2014, vol. 6, no. 4, pp STATISTICAL ANALYSIS OF ATOMIC COLLISIONS DURING METAL VAPOUR NUCLEATION IN NOBEL GAS MEDIUM 1 A.E. Korenchenko 2, A.G. Vorontsov 3, B.R. Gel chinskii 4 The dynamic evaluation of cluster growth probability in supersaturated non-equilibrium medium by statistical analysis of molecular-dynamics calculations was made. The molecular dynamics simulation of copper vapour condensation in argon medium was performed. The possibility of using kinetic molecular theory relations for non-equilibrium conditions was tested. The results show that the number of collisions and scattering cross section agree well with classical values for Ar Ar, Ar Cu and Cu Cu pairs. It was found that the mean lifetime of small clusters (n < 15) does not depend on density of Cu and Ar but it depends on temperature. The research resulted in a new algorithm of cluster growth probability. Keywords: metal clusters; nucleation; molecular dynamics. References 1. Korenchenko A.E., Gelchinski B.R. Matematicheskoe modelirovanie protsessa obrazovaniya metallicheskikh nanochastits pri kondensatsii parov rasplavlennogo metalla (Mathematical simulation of metal nanoparticles formation process at condensation of liquid metal vapors). Rasplavi no. 1. pp (in Russ.). 2. Samokhin A.V., Polyakov S.N., Alekseev N.V., Tsvetkov Yu.V. Fizika i khimiya obrabotki metallov no. 6. pp (in Russ.). 3. Becker R. Doring W. The kinetic treatment of nuclear formation in supersaturated vapors. Ann. Phys Vol. 24. p Krasnochtchekov P., Averback R.S Molecular dynamics simulations of cluster nucleation during inert gas condensation. The Journal of Chemical Physics Vol p Brady J.W., Doll J.D., Thompson D.L. Cluster dynamics: A classical trajectory study of A + An? A*n+1. The Journal of Chemical Physics Vol. 71, no. 6. pp / Insepov Z.A., Karatajev E.M., Norman G.E. The kinetics of condensation behind the shock front. Zeitschrift fur Physik D Atoms, Molecules and Clusters Vol. 20, no. 1. pp Gel chinskii B.R., Vorontsov A.G., Korenchenko A.E., Leont ev L.I. Doklady Acad. Nauk Vol. 436, no. 4. pp (in Russ.). 8. Vorontsov A.G., Gel'Chinskii B.R., Korenchenko A.E. Kinetics and Energy States of Nanoclusters in the Initial Stage of Homogeneous Condensation at High Supersaturation Degrees. Journal of Experimental and Theoretical Physics Vol. 115, no. 5. pp DOI: /S Plimpton S. Fast Parallel Algorithms for Short Range Molecular Dynamics. Journal of Computational Physics Vol pp Kesala E. Kuronen A., Nordlund K. Molecular dynamics simulation of pressure dependence of cluster growth in inert gas condensation. Physical Review B Vol. 75, no. 17. pp Matveev A.N. Molekulyarnaya fizika (Molecular Physics). Moscow: Onics Publ p. (in Russ.). Received 15 September Work is supported by program of presidium of RAS. 2 Korenchenko Anna Evgenevna is Dr. Sc. (Physics and Mathematics), Professor, Optic and Spectroscopy Department, South Ural State University. korenchenko@physics.susu.ac.ru 3 Vorontsov Alexander Gennadevich is Cand. Sc. (Physics and Mathematics), Associate Professor, General and Theoretical Physics Department, South Ural State University. sas@physics.susu.ac.ru 4 Gel chinskii Boris Rafailovich is Dr. Sc. (Physics and Mathematics), Professor, Institute of Metallurgy, Ural Branch of RAS, Ekaterinburg. brg@fmp.ru 2014, 6, 4 25
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