Thermoelectrics: A theoretical approach to the search for better materials
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- Τιμοθέα Μοσχοβάκης
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1 Thermoelectrics: A theoretical approach to the search for better materials Jorge O. Sofo Department of Physics, Department of Materials Science and Engineering, and Materials Research Institute Penn State
2 Abram F. Ioffe The basics
3 The devices Raymond Marlow Sept. 24, Oct. 11, 2013
4 The performance T 1 T 2 Q φ = = W φ MAX SIT T T 2 1 ( 2 1) κ I R /2 2 SI( T2 T1) + I R T ZT T2 / T 1 = ( T2 T1) 1+ ZT + 1 Z + T1 ( T T) 2 1 Z = σ S κ 2
5 Conductivity 101 Drude et al. σ = e 2 n m τ -q q
6 Conductivity 101 y x J = e f ( ) 0 ε v = 0 J = e f v 0
7 f f f H H + = t p r r p f t f {, } H f = t coll d dt ρ 1 i ( t) = H + H ( t), ρ ( t)
8 f f f f dr d + + = t dt r dt t coll
9 f f f f dr d + + = t dt r dt t coll f t = 0 f r = 0
10 d dt f f = t coll
11 d dt f f = t coll d 1 dp ee = = dt dt
12 d dt f f = t coll d 1 dp ee = = dt dt ( ε ) ( ε ) ( ε ) f f ε f = = ε ε v
13 d dt f f = t coll d 1 dp ee = = dt dt f t ( ε ) ( ε ) ( ε ) f f ε f ( ε ) 0 coll = = = ε ε f f τ v
14 d dt f f = t coll d 1 dp ee = = dt dt f t ( ε ) ( ε ) ( ε ) f f ε f ( ε ) 0 coll = = = ε ε f f τ v ( ) f 0 f = f 0 ε + e τ v E ε
15 d dt f f = t coll d 1 dp ee = = dt dt f t ( ε ) ( ε ) ( ε ) f f ε f ( ε ) 0 coll = = = ε ε f f τ v ( ) f 0 f = f 0 ε + e τ v E ε
16 ( ) f 0 f = f 0 ε + e τ v E ε
17 J = e f v ( ) f 0 f = f 0 ε + e τ v E ε
18 0 0 ( ) f f f e v E ε τ ε = + J e f v = 2 0 f J e vv E τ ε =
19 0 0 ( ) f f f e v E ε τ ε = + J e f v = 2 0 f J e vv E τ ε = E J = σ Ω
20 J Ω = σ J = e f v ( ) f 0 f = f 0 ε + e τ v E ε E f 2 0 J= e τ vv E ε σ = e f 2 0 τ vv ε
21 S σ = e κ e f J = σ E σs T J = σst E κ T Q τ v ε B = σ f ε τ v 0 2 ( ε µ ) T B ( ε µ ) 2 f = τ v el B ε T B Z = κ σ 0 el + S 2 κ κ κ σ ph 0 2 el = el ST
22 e 2 f f0 σ = e τ v = e dε Σ( ε) ε ε ( ε ) µ eb f ( ε µ ) ( ) f B S = τ v = dε Σ ε σ ε T B σ ε B T 2 2 ( ε ) µ f ( ε µ ) () 2 f κel = B τ v = B dε Σ ε ε T B ε T B Σ = 2 ( ε) τ vδε ( ε) Transport distribution σ[ Σ ] S[ Σ] κel [ Σ]
23 2 f0 σ = e ( ε ) ε Σ dε S κ el ( ) B f0 ε µ = Σ( ε ) dε σ ε T B Z 2 = σ S Z[ ] 0 κ + κ = Σ Σ best el ph ( ε µ ) 2 2 f0 = B Σ( ε ) ε T B ( ε ) = Cδ ( ε ε 0) dε Σ max Z[ Σ ] = Z[ Σ ] best Σ T ε B The best thermoelectric, G. D. Mahan and J. O. Sofo Proc. Nat. Acad. Sci. USA, 93, 7436 (1996) best
24 The Best Thermoelectric ) ( ) ( ε ε δ τ ε = Σ v v ) ( ) ( ) ( 2 ε τ ε ε v N = ) ( ) ( 0 ε ε δ ε = Σ C best T ε B = ds N ε ε 1 ) ( v ε ε = ) (
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29 J. O. Sofo, G. D. Mahan, Thermoelectric figure of merit of superlattices, Appl. Phys. Lett. 65, 2690 (1994).
30 J. O. Sofo, G. D. Mahan, Thermoelectric figure of merit of superlattices, Appl. Phys. Lett. 65, 2690 (1994).
31 Limitations of the Boltzman Equation Method Also nown as the Kinetic Method because of the relation with classical inetic theory f f f f dr d + + = t dt r dt t coll f H f H f f f + = { H, f } t p r r p t t According to Kubo, Toda, and Hashitsume (1) cannot be applied when the mean free path is too short (e.g., amorphous semiconductors) or the frequency of the applied fields is too high. However, it is very powerful and can be applied to non linear problems. coll (1) R. Kubo, M. Toda, and N. Hashitsume, Statistical Physics II: Non-equilibrium Statistical Mechanics (Springer-Verlag, Berlin, 1991) p. 197
32 Using Boltzman with ab-initio f 0 σ 2 = e ε τ τ v v v 1 ε 1 = p = pˆ m m C. Ambrosch-Draxl and J. O. Sofo Linear optical properties of solids within the full-potential linearized augmented planewave method Comp. Phys. Commun. 175, 1-14 (2006)
33 q q τ First Born Approximation Defect scattering Crystal defects Impurities Neutral Ionized Alloy Carrier-carrier scattering Lattice scattering Intravalley Acoustic Deformation potential Piezoelectric Optic Non-polar Polar Intervalley Acoustic Optic
34 B. R. Nag Electron Transport in Compound Semiconductors
35 B. R. Nag Electron Transport in Compound Semiconductors
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37 T. J. Scheidemantel, C. Ambrosch-Draxl, T. Thonhauser, J. V. Badding, and J. O. Sofo. Transport Coefficients from First-principles Calculations. Phys. Rev. B 68, (2003) Bi 2 Te 3
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39 Georg Madsen s
40 Careful Doping: rigid band Gap problem Temperature dependence of the electronic structure. Alloys. Single site approximations do not wor. Many -points Correlated materials? Connection with magnetism and topology?
41 Linear Response Theory (Kubo) Valid only close to equilibrium 2 i ne σαβ ω δαβ αβ ω ω m 0 ( ) ( + q, = +Π q, + 0 ) β 1 iωτ n Π αβ ( qi, ωn ) = dτe Tj τ α ( q, τ) jβ ( q, τ) V 0 However Does not need well defined energy bands It is easy to incorporate most low energy excitations of the solid Amenable to diagrammatic expansions and controlled approximations Equivalent to the Boltzmann equation when both are valid.
42 Summary Loo for narrow transmission channels with high velocity Tool to explore new compounds, pressure, negative pressure. Prediction of a new compound by G. Madsen. Easy to expand adding new Scattering Mechanisms Limited to applications on non-correlated semiconductors. Magneto-Thermoelectric effects are beginning to be explored.
43 A final comment: EXPERIMENT<-> SIMULATION<->THEORY
44 Simulations describe complexity. Our theoretical wor is to mae it simple
45 Than you! Z 2 = σ S Z[ ] 0 κ + κ = Σ el ph Σ = 2 ( ε) τ vδε ( ε) Transport distribution
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